The DOI matches its Crossref record; 39 of the 39 references it cites were found in a registry or an index.
High‐Entropy Atomic Layers of Transition‐Metal Carbides (MXenes)
Abstract
High‐entropy materials (HEMs) have great potential for energy storage and conversion due to their diverse compositions, and unexpected physical and chemical features. However, high‐entropy atomic layers with fully exposed active sites are difficult to synthesize since their phases are easily segregated. Here, it is demonstrated that high‐entropy atomic layers of transition‐metal carbide (HE‐MXene) can be produced via the selective etching of novel high‐entropy MAX (also termed Mn+1 AXn (n = 1, 2, 3), where M represents an early transition‐metal element, A is an element mainly from groups 13–16, and X stands for C and/or N) phase (HE‐MAX) (Ti 1/5 V 1/5 Zr 1/5 Nb 1/5 Ta 1/5)2 AlC, in which the five transition‐metal species are homogeneously dispersed into one MX slab due to their solid‐solution feature, giving rise to a stable transition‐metal carbide in the atomic layers owing to the high molar configurational entropy and correspondingly low Gibbs free energy. Additionally, the resultant high‐entropy MXene with distinct lattice distortions leads to high mechanical strain into the atomic layers. Moreover, the mechanical strain can efficiently guide the nucleation and uniform growth of dendrite‐free lithium on HE‐MXene, achieving a long cycling stability of up to 1200 h and good deep stripping–plating levels of up to 20 mAh cm−2.
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Cited by
Ten Years of Progress in the Synthesis and Development of MXenes
Naguib, M., Barsoum, M. W., & Gogotsi, Y. (2021) · Advanced Materials · doi:10.1002/adma.202103393 · Cited by 1,257
High-entropy nanoparticles: Synthesis-structure-property relationships and data-driven discovery
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High Entropy van der Waals Materials
Ying, T., Yu, T., Qi, Y., Chen, X., & Hosono, H. (2022) · Advanced Science · doi:10.1002/advs.202203219 · Cited by 51
Metadata
- Authors
- Du, Z., Wu, C., Chen, Y., Cao, Z., Hu, R., Zhang, Y., Gu, J., Cui, Y., Chen, H., Shi, Y., Shang, J., Li, B., & Yang, S.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2021-08-08
- Volume
- 33
- Issue
- 39
- Pages
- e2101473-e2101473
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3191426417
- Cited by
- 322
- References
- 39
- FWCI
- 13.89
- Type
- journal article
- Language
- en
- Open access
- closed
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- Du, Z., Wu, C., Chen, Y., Cao, Z., Hu, R., Zhang, Y., Gu, J., Cui, Y., Chen, H., Shi, Y., Shang, J., Li, B., & Yang, S. (2021). High‐Entropy Atomic Layers of Transition‐Metal Carbides (MXenes). Advanced Materials. https://doi.org/10.1002/adma.202101473
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