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Fast and Long‐Lasting Iron(III) Reduction by Boron Toward Green and Accelerated Fenton Chemistry
Abstract
Generation of hydroxyl radicals in the Fenton system (Fe II/H 2 O 2) is seriously limited by the sluggish kinetics of Fe III reduction and fast Fe III precipitation. Here, boron crystals (C‐Boron) remarkably accelerate the Fe III/Fe II circulation in Fenton‐like systems (C‐Boron/Fe III/H 2 O 2) to produce a myriad of hydroxyl radicals with excellent efficiencies in oxidative degradation of various pollutants. The surface B−B bonds and interfacial suboxide boron in the surface B 12 icosahedra are the active sites to donate electrons to promote fast Fe III reduction to Fe II and further enhance hydroxyl radical production via Fenton chemistry. The C‐Boron/Fe III/H 2 O 2 system outperforms the benchmark Fenton (Fe II/H 2 O 2) and Fe III‐based sulfate radical systems. The reactivity and stability of crystalline boron is much higher than the popular molecular reducing agents, nanocarbons, and other metal/metal‐free nanomaterials.
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Buxton, G. V., Greenstock, C. L., Helman, W. P., & Ross, A. B. (1988) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555805 · Cited by 12,332
Pignatello, J. J., Oliveros, E., & MacKay, A. (2006) · Critical Reviews in Environmental Science and Technology · doi:10.1080/10643380500326564 · Cited by 4,133
Cited by
Defects on CoS2−x: Tuning Redox Reactions for Sustainable Degradation of Organic Pollutants
Ji, J., Yan, Q., Yin, P., Mine, S., Matsuoka, M., & Xing, M. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202013015 · Cited by 280
Metadata
- Authors
- Zhou, P., Ren, W., Nie, G., Li, X., Duan, X., Zhang, Y., & Wang, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-08-13
- Volume
- 59
- Issue
- 38
- Pages
- 16517-16526
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3039403738
- Cited by
- 354
- References
- 2
- FWCI
- 14.35
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhou, P., Ren, W., Nie, G., Li, X., Duan, X., Zhang, Y., & Wang, S. (2020). Fast and Long‐Lasting Iron(III) Reduction by Boron Toward Green and Accelerated Fenton Chemistry. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202007046
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