The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
Proton Capture Strategy for Enhancing Electrochemical CO2 Reduction on Atomically Dispersed Metal–Nitrogen Active Sites**
Abstract
Electrocatalysts play a key role in accelerating the sluggish electrochemical CO 2 reduction (ECR) involving multi‐electron and proton transfer. We now develop a proton capture strategy by accelerating the water dissociation reaction catalyzed by transition‐metal nanoparticles (NPs) adjacent to atomically dispersed and nitrogen‐coordinated single nickel (Ni−Nx) active sites to accelerate proton transfer to the latter for boosting the intermediate protonation step, and thus the whole ECR process. Aberration‐corrected scanning transmission electron microscopy, X‐ray absorption spectroscopy, and calculations reveal that the Ni NPs accelerate the adsorbed H (H ad) generation and transfer to the adjacent Ni−Nx sites for boosting the intermediate protonation and the overall ECR processes. This proton capture strategy is universal to design and prepare for various high‐performance catalysts for diverse electrochemical reactions even beyond ECR.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
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Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
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Exclusive Ni–N4 Sites Realize Near-Unity CO Selectivity for Electrochemical CO2 Reduction
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Cited by
Descriptors for the Evaluation of Electrocatalytic Reactions: d‐Band Theory and Beyond
Jiao, S., Fu, X., & Huang, H. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202107651 · Cited by 719
Fu, H. Q., Zhou, M., Liu, P. F., Liu, P., Yin, H., Sun, K. Z., Yang, H. G., Al-Mamun, M., Hu, P., Wang, H.-F., et al. (2022) · Journal of the American Chemical Society · doi:10.1021/jacs.2c01094 · Cited by 508
Wang, K., Cao, J., Yang, X., Sang, X., Yao, S., Xiang, R., Yang, B., Li, Z., O'Carroll, T., Zhang, Q., et al. (2023) · Advanced Functional Materials · doi:10.1002/adfm.202212321 · Cited by 98
Self-citation
Metadata
- Authors
- Wang, X., Sang, X., Dong, C., Yao, S., Shuai, L., Lu, J., Yang, B., Li, Z., Lei, L., Qiu, M., Dai, L., & Hou, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-04-12
- Volume
- 60
- Issue
- 21
- Pages
- 11959-11965
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3120746273
- Cited by
- 267
- References
- 37
- FWCI
- 9.01
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, X., Sang, X., Dong, C., Yao, S., Shuai, L., Lu, J., Yang, B., Li, Z., Lei, L., Qiu, M., Dai, L., & Hou, Y. (2021). Proton Capture Strategy for Enhancing Electrochemical CO2 Reduction on Atomically Dispersed Metal–Nitrogen Active Sites**. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202100011
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