The DOI matches its Crossref record; 48 of the 48 references it cites were found in a registry or an index.
Regulative Electronic States around Ruthenium/Ruthenium Disulphide Heterointerfaces for Efficient Water Splitting in Acidic Media
Abstract
Theoretical calculations unveil the charge redistribution over abundant interfaces and the enhanced electronic states of Ru/RuS 2 heterostructure. The resulting surface electron‐deficient Ru sites display optimized adsorption behavior toward diverse reaction intermediates, thereby reducing the thermodynamic energy barriers. Experimentally, for the first time the laminar Ru/RuS 2 heterostructure is rationally engineered by virtue of the synchronous reduction and sulfurization under eutectic salt system. Impressively, it exhibits extremely high catalytic activity for both OER (201 mV @ 10 mA cm−2) and HER (45 mV @ 10 mA cm−2) in acidic media due to favorable kinetics and excellent specific activity, consequently leading to a terrific performance in acidic overall water splitting devices (1.501 V @ 10 mA cm−2). The in‐depth insight into the internal activity origin of interfacial effect could offer precise guidance for the rational establishment of hybrid interfaces.
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Self-citationZhu, Y. P., Guo, C., Zheng, Y., & Qiao, S.-Z. (2017) · Accounts of Chemical Research · doi:10.1021/acs.accounts.6b00635 · Cited by 1,026
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Cited by
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Hydrogen production by water electrolysis technologies: A review
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Wang, Y., Yang, R., Ding, Y., Zhang, B., Li, H., Bai, B., Li, M., Cui, Y., Xiao, J., & Wu, Z.-S. (2023) · Nature Communications · doi:10.1038/s41467-023-37008-8 · Cited by 547
PEM water electrolysis for hydrogen production: fundamentals, advances, and prospects
Wang, T., Cao, X., & Jiao, L. (2022) · Carbon Neutrality · doi:10.1007/s43979-022-00022-8 · Cited by 389
Metadata
- Authors
- Zhu, J., Guo, Y., Liu, F., Xu, H., Gong, L., Shi, W., Chen, D., Wang, P., Yang, Y., Zhang, C., Wu, J., Luo, J., & Mu, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-03-30
- Volume
- 60
- Issue
- 22
- Pages
- 12328-12334
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3129275027
- Cited by
- 293
- References
- 48
- FWCI
- 9.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhu, J., Guo, Y., Liu, F., Xu, H., Gong, L., Shi, W., Chen, D., Wang, P., Yang, Y., Zhang, C., Wu, J., Luo, J., & Mu, S. (2021). Regulative Electronic States around Ruthenium/Ruthenium Disulphide Heterointerfaces for Efficient Water Splitting in Acidic Media. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202101539
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