The DOI matches its Crossref record; 19 of the 19 references it cites were found in a registry or an index.
Particulate Photocatalysts for Light-Driven Water Splitting: Mechanisms, Challenges, and Design Strategies
Abstract
Solar-driven water splitting provides a leading approach to store the abundant yet intermittent solar energy and produce hydrogen as a clean and sustainable energy carrier. A straightforward route to light-driven water splitting is to apply self-supported particulate photocatalysts, which is expected to allow solar hydrogen to be competitive with fossil-fuel-derived hydrogen on a levelized cost basis. More importantly, the powder-based systems can lend themselves to making functional panels on a large scale while retaining the intrinsic activity of the photocatalyst. However, all attempts to generate hydrogen via powder-based solar water-splitting systems to date have unfortunately fallen short of the efficiency values required for practical applications. Photocatalysis on photocatalyst particles involves three sequential steps: (i) absorption of photons with higher energies than the bandgap of the photocatalysts, leading to the excitation of electron-hole pairs in the particles, (ii) charge separation and migration of these photoexcited carriers, and (iii) surface chemical reactions based on these carriers. In this review, we focus on the challenges of each step and summarize material design strategies to overcome the obstacles and limitations. This review illustrates that it is possible to employ the fundamental principles underlying photosynthesis and the tools of chemical and materials science to design and prepare photocatalysts for overall water splitting.
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Challenges for photocatalytic overall water splitting
Bie, C., Wang, L., & Yu, J. (2022) · Chem · doi:10.1016/j.chempr.2022.04.013 · Cited by 874
Conquering the Hypoxia Limitation for Photodynamic Therapy
Wan, Y., Fu, L., Li, C., Lin, J., & Huang, P. (2021) · Advanced Materials · doi:10.1002/adma.202103978 · Cited by 705
Emerging Cocatalysts on g‐C3N4 for Photocatalytic Hydrogen Evolution
Zhu, Q., Xu, Z., Qiu, B., Xing, M., & Zhang, J. (2021) · Small · doi:10.1002/smll.202101070 · Cited by 380
Xu, M., Li, D., Sun, K., Jiao, L., Xie, C., Ding, C., & Jiang, H. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202104219 · Cited by 280
Metadata
- Authors
- Wang, Q., & Domen, K.
- Venue
- Chemical Reviews
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-08-08
- Volume
- 120
- Issue
- 2
- Pages
- 919-985
- ISSN
- 0009-2665 (ISSN-L)
- 1520-6890
- OpenAlex
- W2967197658
- Cited by
- 2,809
- References
- 19
- FWCI
- 9.53
- Type
- journal article
- Language
- en
- Open access
- closed
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