The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Ether‐Based Electrolyte Chemistry Towards High‐Voltage and Long‐Life Na‐Ion Full Batteries
Abstract
Although ether‐based electrolytes have been extensively applied in anode evaluation of batteries, anodic instability arising from solvent oxidability is always a tremendous obstacle to matching with high‐voltage cathodes. Herein, by rational design for solvation configuration, the fully coordinated ether‐based electrolyte with strong resistance against oxidation is reported, which remains anodically stable with high‐voltage Na 3 V 2(PO 4)2 O 2 F (NVPF) cathode under 4.5 V (versus Na+/Na) protected by an effective interphase. The assembled graphite//NVPF full cells display superior rate performance and unprecedented cycling stability. Beyond that, the constructed full cells coupling the high‐voltage NVPF cathode with hard carbon anode exhibit outstanding electrochemical performances in terms of high average output voltage up to 3.72 V, long‐term cycle life (such as 95 % capacity retention after 700 cycles) and high energy density (247 Wh kg−1). In short, the optimized ether‐based electrolyte enriches systematic options, the ability to maintain oxidative stability and compatibility with various anodes, exhibiting attractive prospects for application.
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Citations
Cites
Tailoring electrolyte solvation for Li metal batteries cycled at ultra-low temperature
Holoubek, J., Liu, H., Wu, Z., Yin, Y., Xing, X., Cai, G., Yu, S., Zhou, H., Pascal, T. A., Chen, Z., et al. (2021) · Nature Energy · doi:10.1038/s41560-021-00783-z · Cited by 851
Cited by
Emerging Era of Electrolyte Solvation Structure and Interfacial Model in Batteries
Cheng, H., Sun, Q., Li, L., Zou, Y., Wang, Y., Cai, T., Zhao, F., Liu, G., Ma, Z., Wahyudi, W., et al. (2022) · ACS Energy Letters · doi:10.1021/acsenergylett.1c02425 · Cited by 640
A 30‐year overview of sodium‐ion batteries
Gao, Y., Zhang, H., Peng, J., Li, L., Xiao, Y., Li, L., Liu, Y., Qiao, Y., & Chou, S. (2024) · Carbon Energy · doi:10.1002/cey2.464 · Cited by 348
Electrolytes in Organic Batteries
Li, M., Hicks, R. P., Chen, Z., Luo, C., Guo, J., Wang, C., & Xu, Y. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00374 · Cited by 303
Self-citationElectrolyte design implications of ion-pairing in low-temperature Li metal batteries
Holoubek, J., Kim, K., Yin, Y., Wu, Z., Liu, H., Li, M., Chen, A., Gao, H., Cai, G., Pascal, T. A., et al. (2022) · Energy & Environmental Science · doi:10.1039/d1ee03422g · Cited by 241
He, J., Tao, T., Yang, F., & Sun, Z. (2022) · ChemSusChem · doi:10.1002/cssc.202102522 · Cited by 29
Metadata
- Authors
- Liang, H., Gu, Z., Zhao, X., Guo, J., Yang, J., Li, W., Li, B., Liu, Z., Li, W., & Wu, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-11-15
- Volume
- 60
- Issue
- 51
- Pages
- 26837-26846
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3205790928
- Cited by
- 301
- References
- 1
- FWCI
- 14.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liang, H., Gu, Z., Zhao, X., Guo, J., Yang, J., Li, W., Li, B., Liu, Z., Li, W., & Wu, X. (2021). Ether‐Based Electrolyte Chemistry Towards High‐Voltage and Long‐Life Na‐Ion Full Batteries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202112550
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