The DOI matches its Crossref record; 64 of the 64 references it cites were found in a registry or an index.
Manipulating the Water Dissociation Electrocatalytic Sites of Bimetallic Nickel‐Based Alloys for Highly Efficient Alkaline Hydrogen Evolution
Abstract
Transition‐metal alloys are currently drawing increasing attention as promising electrocatalysts for the alkaline hydrogen evolution reaction (HER). However, traditional density‐functional‐theory‐derived d‐band theory fails to describe the hydrogen adsorption energy (Δ GH) on hollow sites. Herein, by studying the Δ GH for a series of Ni−M (M=Ti, V, Cr, Mn, Fe, Co, Cu, Zn, Mo, W) bimetallic alloys, an improved d‐band center was provided and a potential NiCu electrocatalyst with a near‐optimal Δ GH was discovered. Moreover, oxygen atoms were introduced into Ni−M (O−NiM) to balance the adsorption/desorption of hydroxyl species. The tailored electrocatalytic sites for water dissociation can synergistically accelerate the multi‐step alkaline HER. The prepared O−NiCu shows the optimum HER activity with a low overpotential of 23 mV at 10 mA cm−2. This work not only broadens the applicability of d‐band theory, but also provides crucial understanding for designing efficient HER electrocatalysts.
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Cited by
Gao, G., Zhu, G., Chen, X., Sun, Z., & Cabot, A. (2023) · ACS Nano · doi:10.1021/acsnano.3c05810 · Cited by 278
Computational chemistry for water-splitting electrocatalysis
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Wu, Z., Yang, P., Li, Q., Xiao, W., Li, Z., Xu, G., Liu, F., Jia, B., Ma, T., Feng, S., et al. (2023) · Angewandte Chemie International Edition · doi:10.1002/anie.202300406 · Cited by 226
Self-citationAn ultra-low Pt metal nitride electrocatalyst for sustainable seawater hydrogen production
Hu, H., Zhang, Z., Zhang, Y., Thomas, T., Du, H., Huang, K., Attfield, J. P., & Yang, M. (2023) · Energy & Environmental Science · doi:10.1039/d3ee01541f · Cited by 161
Self-citationHou, L., Li, C., Jang, H., Kim, M. G., Jiang, J., Cho, J., Liu, S., & Liu, X. (2024) · Advanced Materials · doi:10.1002/adma.202410039 · Cited by 126
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Metadata
- Authors
- Wang, J., Xin, S., Xiao, Y., Zhang, Z., Li, Z., Zhang, W., Li, C., Bao, R., Peng, J., Yi, J., & Chou, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-06-09
- Volume
- 61
- Issue
- 30
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4225562089
- Cited by
- 303
- References
- 64
- FWCI
- 11.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, J., Xin, S., Xiao, Y., Zhang, Z., Li, Z., Zhang, W., Li, C., Bao, R., Peng, J., Yi, J., & Chou, S. (2022). Manipulating the Water Dissociation Electrocatalytic Sites of Bimetallic Nickel‐Based Alloys for Highly Efficient Alkaline Hydrogen Evolution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202202518
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