The DOI matches its Crossref record; 36 of the 36 references it cites were found in a registry or an index.
High‐Entropy Prussian Blue Analogues and Their Oxide Family as Sulfur Hosts for Lithium‐Sulfur Batteries
Abstract
The introduction of high‐entropy into Prussian blue analogues (PBAs) has yet to attract attention in the field of lithium‐sulfur battery materials. Herein, we systematically synthesize a library of PBAs from binary to high‐entropy by a facile coprecipitation method. The coordination environment in PBAs is explored by X‐ray absorption fine structure spectroscopy, which together with elemental mapping confirm the successful introduction of all metals. Importantly, electrochemical tests demonstrate that high‐entropy PBA can serve as polysulfide immobilizer to inhibit shuttle effect and as catalyst to promote polysulfides conversion, thereby boosting its outstanding performance. Additionally, a variety of nanocubic metal oxides from binary to senary are fabricated by using PBAs as sacrificial precursors. We believe that a wide range of new materials obtained from our coprecipitation and pyrolysis methodology can promote further developments in research on PBA systems and sulfur hosts.
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Cites
Fei, H., Dong, J., Feng, Y., Allen, C. S., Wan, C., Volosskiy, B., Li, M., Zhao, Z., Wang, Y., Sun, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0008-y · Cited by 1,973
High entropy oxides for reversible energy storage
Sarkar, A., Velasco, L., Wang, D., Wang, Q., Talasila, G., de Biasi, L., Kübel, C., Brezesinski, T., Bhattacharya, S. S., Hahn, H., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-05774-5 · Cited by 1,351
Shang, H., Zhou, X., Dong, J., Li, A., Zhao, X., Liu, Q., Lin, Y., Pei, J., Li, Z., Jiang, Z., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-16848-8 · Cited by 929
Prussian Blue Cathode Materials for Sodium‐Ion Batteries and Other Ion Batteries
Qian, J., Wu, C., Cao, Y., Ma, Z., Huang, Y., Ai, X., & Yang, H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702619 · Cited by 871
Prussian Blue Analogs as Battery Materials
Hurlbutt, K., Wheeler, S., Capone, I., & Pasta, M. (2018) · Joule · doi:10.1016/j.joule.2018.07.017 · Cited by 726
(2020) · doi:10.1038/s41467-020-19277-9 · Cited by 690
Duan, Y., Yu, Z., Hu, S., Zheng, X., Zhang, C., Ding, H., Hu, B., Fu, Q., Yu, Z., Zheng, X., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201909939 · Cited by 625
Zheng, S., Li, Q., Xue, H., Pang, H., & Xü, Q. (2019) · National Science Review · doi:10.1093/nsr/nwz137 · Cited by 625
Self-citationRecent progress of high-entropy materials for energy storage and conversion
Amiri, A., & Shahbazian-Yassar, R. (2021) · Journal of Materials Chemistry A · doi:10.1039/d0ta09578h · Cited by 592
Pan, Y., Sun, K., Lin, Y., Cao, X., Cheng, Y., Liu, S., Zeng, L., Cheong, W.-C., Zhao, D., Wu, K., et al. (2019) · Nano Energy · doi:10.1016/j.nanoen.2018.11.034 · Cited by 567
Metadata
- Authors
- Du, M., Geng, P., Pei, C., Jiang, X., Shan, Y., Hu, W., Ni, L., & Pang, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-09-08
- Volume
- 61
- Issue
- 41
- Pages
- e202209350-e202209350
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4293105509
- Cited by
- 428
- References
- 36
- FWCI
- 24.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Du, M., Geng, P., Pei, C., Jiang, X., Shan, Y., Hu, W., Ni, L., & Pang, H. (2022). High‐Entropy Prussian Blue Analogues and Their Oxide Family as Sulfur Hosts for Lithium‐Sulfur Batteries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202209350
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