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High entropy oxides for reversible energy storage
Open accessAbstract
In recent years, the concept of entropy stabilization of crystal structures in oxide systems has led to an increased research activity in the field of “high entropy oxides”. These compounds comprise the incorporation of multiple metal cations into single-phase crystal structures and interactions among the various metal cations leading to interesting novel and unexpected properties. Here, we report on the reversible lithium storage properties of the high entropy oxides, the underlying mechanisms governing these properties, and the influence of entropy stabilization on the electrochemical behavior. It is found that the stabilization effect of entropy brings significant benefits for the storage capacity retention of high entropy oxides and greatly improves the cycling stability. Additionally, it is observed that the electrochemical behavior of the high entropy oxides depends on each of the metal cations present, thus providing the opportunity to tailor the electrochemical properties by simply changing the elemental composition.
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Citations
Cited by
George, E. P., Raabe, D., & Ritchie, R. O. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0121-4 · Cited by 5,047
Oses, C., Toher, C., & Curtarolo, S. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0170-8 · Cited by 2,081
High-entropy energy materials: challenges and new opportunities
Ma, Y., Ma, Y., Wang, Q., Schweidler, S., Botros, M., Fu, T., Hahn, H., Brezesinski, T., & Breitung, B. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00505g · Cited by 963
Self-citationReview of high entropy ceramics: design, synthesis, structure and properties
Zhang, R.-Z., & Reece, M. J. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta05698j · Cited by 760
Cation-disordered rocksalt-type high-entropy cathodes for Li-ion batteries
Lun, Z., Ouyang, B., Kwon, D.-H., Ha, Y., Foley, E. E., Huang, T.-Y., Cai, Z., Kim, H., Balasubramanian, M., Sun, Y., et al. (2021) · Nature Materials · doi:10.1038/s41563-020-00816-0 · Cited by 689
Metadata
- Authors
- Sarkar, A., Velasco, L., Wang, D., Wang, Q., Talasila, G., de Biasi, L., Kübel, C., Brezesinski, T., Bhattacharya, S. S., Hahn, H., & Breitung, B.
- Venue
- Nature Communications
- Published
- 2018-08-24
- Volume
- 9
- Issue
- 1
- Pages
- 3400-3400
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2888579709
- Cited by
- 1,351
- References
- 0
- FWCI
- 22.96
- Type
- journal article
- Language
- en
- Open access
- gold
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- Sarkar, A., Velasco, L., Wang, D., Wang, Q., Talasila, G., de Biasi, L., Kübel, C., Brezesinski, T., Bhattacharya, S. S., Hahn, H., & Breitung, B. (2018). High entropy oxides for reversible energy storage. Nature Communications. https://doi.org/10.1038/s41467-018-05774-5
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