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Mechanism of Lithium Storage in MoS2 and the Feasibility of Using Li2S/Mo Nanocomposites as Cathode Materials for Lithium–Sulfur Batteries
Abstract
The most‐popular strategy to improve the cycling stability and rate performance of the sulfur electrode in lithium–sulfur (Li–S) batteries is to astrict the sulfur in a conducting medium by using complicated chemical/physical processing. Lithium sulfide (Li 2 S) has been proposed as an alternative electrode material to sulfur. However, for its application, it must meet challenges such as high instability in air together with all of the drawbacks of a sulfur–containing electrode. Herein, we report the feasibility of using Li 2 S, which was obtained by electrochemical conversion of commercial molybdenum disulfide (MoS 2) into Li 2 S and metallic molybdenium (Mo) at low voltages, as a high‐performance active material in Li–S batteries. Metallic Mo prevented the dissolution of lithium polysulfides into the electrolyte and enhanced the conductivity of the sulfide electrode. Therefore, the in situ electrochemically prepared Li 2 S/Mo composite exhibited both high cycling stability and high sulfur utilization.
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Cited by
Electrode Degradation in Lithium-Ion Batteries
Pender, J. P., Jha, G., Youn, D. H., Ziegler, J. M., Andoni, I., Choi, E. J., Heller, A., Dunn, B. S., Weiss, P. S., Penner, R. M., et al. (2020) · ACS Nano · doi:10.1021/acsnano.9b04365 · Cited by 873
Nanostructured Mo-based electrode materials for electrochemical energy storage
Hu, X., Zhang, W., Liu, X., Mei, Y., & Huang, Y. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00350k · Cited by 711
Wang, J., Liu, J., Chao, D., Yan, J., Lin, J., & Shen, Z. X. (2014) · Advanced Materials · doi:10.1002/adma.201402728 · Cited by 442
Synthesis of MoS2 nanosheet–graphene nanosheet hybrid materials for stable lithium storage
Zhou, X., Wan, L.-J., & Guo, Y.-G. (2013) · Chemical Communications · doi:10.1039/c3cc38780a · Cited by 304
Metadata
- Authors
- Fang, X., Guo, X., Mao, Y., Hua, C., Shen, L., Hu, Y., Wang, Z., Wu, F., & Chen, L.
- Venue
- Chemistry – An Asian Journal
- Publisher
- Wiley
- Published
- 2012-02-28
- Volume
- 7
- Issue
- 5
- Pages
- 1013-1017
- ISSN
- 1861-471X (ISSN-L)
- 1861-4728
- OpenAlex
- W2132704987
- Cited by
- 168
- References
- 0
- FWCI
- 11.19
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fang, X., Guo, X., Mao, Y., Hua, C., Shen, L., Hu, Y., Wang, Z., Wu, F., & Chen, L. (2012). Mechanism of Lithium Storage in MoS2 and the Feasibility of Using Li2S/Mo Nanocomposites as Cathode Materials for Lithium–Sulfur Batteries. Chemistry – An Asian Journal. https://doi.org/10.1002/asia.201100796
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