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Adsorption of Polycyclic Aromatic Hydrocarbons on Graphene Oxides and Reduced Graphene Oxides
Abstract
Graphene has attracted increasing attention in multidisciplinary studies because of its unique physical and chemical properties. Herein, the adsorption of polycyclic aromatic hydrocarbons (PAHs), such as naphthalene (NAP), anthracene (ANT), and pyrene (PYR), on reduced graphene oxides (rGOs) and graphene oxides (GOs) as a function of pH, humic acid (HA), and temperature were elucidated by means of a batch technique. For comparison, nonpolar and nonporous graphite were also employed in this study. The increasing of pH from 2 to 11 did not influence the adsorption of PAHs on rGOs, whereas the suppressed adsorption of NAP on rGOs was observed both in the presence of HA and under high‐temperature conditions. Adsorption isotherms of PAHs on rGOs were in accordance with the Polanyi–Dubinin–Ashtahhov (PDA) model, providing evidence that pore filling and flat surface adsorption were involved. The saturated adsorbed capacities (in mmol g−1) of rGOs for PAHs calculated from the PDA model significantly decreased in the order of NAP>PYR>ANT, which was comparable to the results of theoretical calculations. The pore‐filling mechanism dominates the adsorption of NAP on rGOs, but the adsorption mechanisms of ANT and PYR on rGOs are flat surface adsorption.
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Cites
Quantifying the Total and Bioavailable Polycyclic Aromatic Hydrocarbons and Dioxins in Biochars
Hale, S. E., Lehmann, J., Rutherford, D., Zimmerman, A. R., Bachmann, R. T., Shitumbanuma, V., O’Toole, A., Sundqvist, K. L., Arp, H. P. H., & Cornelissen, G. (2012) · Environmental Science & Technology · doi:10.1021/es203984k · Cited by 634
Cited by
Jin, Z., Wang, X., Sun, Y., Ai, Y., & Wang, X. (2015) · Environmental Science & Technology · doi:10.1021/acs.est.5b02022 · Cited by 477
Self-citationGraphene and Graphene Oxide-Based Composites for Removal of Organic Pollutants: A Review
Thakur, K., & Kandasubramanian, B. (2019) · Journal of Chemical & Engineering Data · doi:10.1021/acs.jced.8b01057 · Cited by 469
Kong, Q., Shi, X., Ma, W., Zhang, F., Yu, T., Zhao, F., Zhao, D., & Wei, C. (2021) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2021.125690 · Cited by 267
Metadata
- Authors
- Sun, Y., Yang, S., Zhao, G., Wang, Q., & Wang, X.
- Venue
- Chemistry – An Asian Journal
- Publisher
- Wiley
- Published
- 2013-08-12
- Volume
- 8
- Issue
- 11
- Pages
- 2755-2761
- ISSN
- 1861-471X (ISSN-L)
- 1861-4728
- OpenAlex
- W2018917895
- Cited by
- 176
- References
- 1
- FWCI
- 18.63
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sun, Y., Yang, S., Zhao, G., Wang, Q., & Wang, X. (2013). Adsorption of Polycyclic Aromatic Hydrocarbons on Graphene Oxides and Reduced Graphene Oxides. Chemistry – An Asian Journal. https://doi.org/10.1002/asia.201300496
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