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Ionic Conductivity in the Metal–Organic Framework UiO‐66 by Dehydration and Insertion of Lithium tert‐Butoxide
Abstract
Shields up! Post-synthetic modification of the secondary building units in the metal-organic framework UiO-66 (Zr6O4(OH)4(O2CR)12) by dehydration and subsequent grafting of LiOtBu yields a solid Li(+) electrolyte with a conductivity of 1.8×10(-5) S cm(-1) at 293 K. As the grafting leads to screening of the anionic charge, the activation energy for ionic conduction is significantly lower than when Li(+) is introduced through deprotonation.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Zr-based metal–organic frameworks: design, synthesis, structure, and applications
Bai, Y., Dou, Y., Xie, L.-H., Rutledge, W., Li, J.-R., & Zhou, H.-C. (2016) · Chemical Society Reviews · doi:10.1039/c5cs00837a · Cited by 2,545
Metal–organic frameworks for energy storage: Batteries and supercapacitors
Wang, L., Han, Y., Feng, X., Zhou, J., Qi, P., & Wang, B. (2016) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2015.09.002 · Cited by 1,298
Defect‐Engineered Metal–Organic Frameworks
Fang, Z., Bueken, B., De Vos, D. E., & Fischer, R. A. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201411540 · Cited by 1,252
Applications of water stable metal–organic frameworks
Wang, C., Liu, X., Keser Demir, N., Chen, J. P., & Li, K. (2016) · Chemical Society Reviews · doi:10.1039/c6cs00362a · Cited by 1,249
Ionic Covalent Organic Frameworks with Spiroborate Linkage
Du, Y., Yang, H., Whiteley, J. M., Wan, S., Jin, Y., Lee, S., & Zhang, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201509014 · Cited by 674
Metadata
- Authors
- Ameloot, R., Aubrey, M., Wiers, B. M., Gómora‐Figueroa, A. P., Patel, S. N., Balsara, N. P., & Long, J. R.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2013-03-12
- Volume
- 19
- Issue
- 18
- Pages
- 5533-5536
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2142988903
- Cited by
- 222
- References
- 1
- FWCI
- 6.60
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Ionic Conductivity in the Metal–Organic Framework UiO‐66 by Dehydration and Insertion of Lithium tert‐Butoxide. https://app.cochat.ai/papers/10.1002/chem.201300326
- The paper
- Ameloot, R., Aubrey, M., Wiers, B. M., Gómora‐Figueroa, A. P., Patel, S. N., Balsara, N. P., & Long, J. R. (2013). Ionic Conductivity in the Metal–Organic Framework UiO‐66 by Dehydration and Insertion of Lithium tert‐Butoxide. Chemistry – A European Journal. https://doi.org/10.1002/chem.201300326
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