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A Covalent Organic Framework–Cadmium Sulfide Hybrid as a Prototype Photocatalyst for Visible‐Light‐Driven Hydrogen Production
Abstract
CdS nanoparticles were deposited on a highly stable, two‐dimensional (2D) covalent organic framework (COF) matrix and the hybrid was tested for photocatalytic hydrogen production. The efficiency of CdS‐COF hybrid was investigated by varying the COF content. On the introduction of just 1 wt % of COF, a dramatic tenfold increase in the overall photocatalytic activity of the hybrid was observed. Among the various hybrids synthesized, that with 10 wt % COF, named CdS‐COF (90:10), was found to exhibit a steep H 2 production amounting to 3678 μmol h−1 g−1, which is significantly higher than that of bulk CdS particles (124 μmol h−1 g−1). The presence of a π‐conjugated backbone, high surface area, and occurrence of abundant 2D hetero‐interface highlight the usage of COF as an effective support for stabilizing the generated photoelectrons, thereby resulting in an efficient and high photocatalytic activity.
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Cited by
Sulfone-containing covalent organic frameworks for photocatalytic hydrogen evolution from water
Wang, X., Chen, L., Chong, S. Y., Little, M. A., Wu, Y., Zhu, W.-H., Clowes, R., Yan, Y., Zwijnenburg, M. A., Sprick, R. S., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0141-5 · Cited by 1,320
Covalent Organic Framework Photocatalysts: Structures and Applications
Wang, H., Wang, H., Wang, Z., Tang, L., Zeng, G., Xu, P., Chen, M., Xiong, T., Zhou, C., Li, X., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00278j · Cited by 1,301
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Beuerle, F., & Gole, B. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201710190 · Cited by 528
Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges
Pan, H., Li, J., Wang, Y., Xia, Q., Qiu, L., & Zhou, B. (2024) · Advanced Science · doi:10.1002/advs.202402651 · Cited by 67
Metadata
- Authors
- Thote, J., Aiyappa, H. B., Deshpande, A., Díaz Díaz, D., Kurungot, S., & Banerjee, R.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2014-10-13
- Volume
- 20
- Issue
- 48
- Pages
- 15961-15965
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2131710556
- Cited by
- 263
- References
- 0
- FWCI
- 3.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Thote, J., Aiyappa, H. B., Deshpande, A., Díaz Díaz, D., Kurungot, S., & Banerjee, R. (2014). A Covalent Organic Framework–Cadmium Sulfide Hybrid as a Prototype Photocatalyst for Visible‐Light‐Driven Hydrogen Production. Chemistry – A European Journal. https://doi.org/10.1002/chem.201403800
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