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MIL‐101‐SO3H: A Highly Efficient Brønsted Acid Catalyst for Heterogeneous Alcoholysis of Epoxides under Ambient Conditions
Abstract
For the first time, a ∼100 % sulfonic acid functionalized metal–organic framework (MOF), MIL‐101‐SO 3 H, with giant pores has been prepared by a hydrothermal process followed by a facile postsynthetic HCl treatment strategy. The replete readily accessible Lewis acidic and especially Brønsted acidic sites distributed throughout the framework as well as high stability endow the resultant MOF exceptionally high efficiency and recyclability, which surpass all other MOF‐based catalysts, for the ring opening of epoxides with alcohols (especially, methanol) as nucleophiles under ambient conditions.
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Horike, S., Shimomura, S., & Kitagawa, S. (2009) · Nature Chemistry · doi:10.1038/nchem.444 · Cited by 2,486
Cited by
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Yang, Q., Xu, Q., & Jiang, H.-L. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00724d · Cited by 1,892
Self-citationMetal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications
Cai, G., Yan, P., Zhang, L., Zhou, H.-C., & Jiang, H.-L. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00243 · Cited by 1,631
Self-citationCatalysis by Metal Organic Frameworks: Perspective and Suggestions for Future Research
Yang, D., & Gates, B. C. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b04515 · Cited by 932
Metadata
- Authors
- Zhou, Y., Chen, Y., Hu, Y., Huang, G., Yu, S., & Jiang, H.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2014-10-07
- Volume
- 20
- Issue
- 46
- Pages
- 14976-14980
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2127855165
- Cited by
- 180
- References
- 1
- FWCI
- 6.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Zhou, Y., Chen, Y., Hu, Y., Huang, G., Yu, S., & Jiang, H. (2014). MIL‐101‐SO3H: A Highly Efficient Brønsted Acid Catalyst for Heterogeneous Alcoholysis of Epoxides under Ambient Conditions. Chemistry – A European Journal. https://doi.org/10.1002/chem.201404104
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