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Measurements of volatile organic compounds in the earth's atmosphere using proton‐transfer‐reaction mass spectrometry
Abstract
Proton‐transfer‐reaction mass spectrometry (PTR‐MS) allows real‐time measurements of volatile organic compounds (VOCs) in air with a high sensitivity and a fast time response. The use of PTR‐MS in atmospheric research has expanded rapidly in recent years, and much has been learned about the instrument response and specificity of the technique in the analysis of air from different regions of the atmosphere. This paper aims to review the progress that has been made. The theory of operation is described and allows the response of the instrument to be described for different operating conditions. More accurate determinations of the instrument response involve calibrations using standard mixtures, and some results are shown. Much has been learned about the specificity of PTR‐MS from inter‐comparison studies as well the coupling of PTR‐MS with a gas chromatographic interface. The literature on this issue is reviewed and summarized for many VOCs of atmospheric interest. Some highlights of airborne measurements by PTR‐MS are presented, including the results obtained in fresh and aged forest‐fire and urban plumes. Finally, the recent work that is focused on improving the technique is discussed. © 2006 Wiley Periodicals, Inc. Mass Spec Rev 26:223–257, 2007
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CRC Handbook of Chemistry and Physics
(2014) · doi:10.1201/b17118 · Cited by 57,706
Holzinger, R., Warneke, C., Hansel, A., Jordan, A., Lindinger, W., Scharffe, D. H., Schade, G., & Crutzen, P. J. (1999) · Geophysical Research Letters · doi:10.1029/1999gl900156 · Cited by 343
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Salthammer, T., Mentese, S., & Marutzky, R. (2010) · Chemical Reviews · doi:10.1021/cr800399g · Cited by 1,808
Schwarz, J. P., Gao, R. S., Spackman, J. R., Watts, L. A., Thomson, D. S., Fahey, D. W., Ryerson, T. B., Peischl, J., Holloway, J. S., Trainer, M., et al. (2008) · Geophysical Research Letters · doi:10.1029/2008gl033968 · Cited by 466
Self-citationWest, J. J., Cohen, A., Dentener, F., Brunekreef, B., Zhu, T., Armstrong, B., Bell, M. L., Brauer, M., Carmichael, G., Costa, D. L., et al. (2016) · Environmental Science & Technology · doi:10.1021/acs.est.5b03827 · Cited by 390
Cappellin, L., Karl, T., Probst, M., Ismailova, O., Winkler, P. M., Soukoulis, C., Aprea, E., Märk, T. D., Gasperi, F., & Biasioli, F. (2012) · Environmental Science & Technology · doi:10.1021/es203985t · Cited by 344
Warneke, C., Bahreini, R., Brioude, J., Brock, C. A., de Gouw, J. A., Fahey, D. W., Froyd, K. D., Holloway, J. S., Middlebrook, A., Miller, L., et al. (2009) · Geophysical Research Letters · doi:10.1029/2008gl036194 · Cited by 260
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Metadata
- Authors
- de Gouw, J., & Warneke, C.
- Venue
- Mass Spectrometry Reviews
- Publisher
- Wiley
- Published
- 2006-12-07
- Volume
- 26
- Issue
- 2
- Pages
- 223-257
- ISSN
- 0277-7037 (ISSN-L)
- 1098-2787
- OpenAlex
- W2047457654
- Cited by
- 1,055
- References
- 2
- FWCI
- 12.72
- Type
- journal article
- Language
- en
- Open access
- closed
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