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Understanding the Photothermal Conversion Efficiency of Gold Nanocrystals
Abstract
Plasmon‐based photothermal therapy is one of the most intriguing applications of noble metal nanostructures. The photothermal conversion efficiency is an essential parameter in practically realizing this application. The effects of the plasmon resonance wavelength, particle volume, shell coating, and assembly on the photothermal conversion efficiencies of Au nanocrystals are systematically studied by directly measuring the temperature of Au nanocrystal solutions with a thermocouple and analyzed on the basis of energy balance. The temperature of Au nanocrystal solutions reaches the maximum at ∼75°C when the plasmon resonance wavelength of Au nanocrystals is equal to the illumination laser wavelength. For Au nanocrystals with similar shapes, the larger the nanocrystal, the smaller the photothermal conversion efficiency becomes. The photothermal conversion can also be controlled by shell coating and assembly through the change in the plasmon resonance energy of Au nanocrystals. Moreover, coating Au nanocrystals with semiconductor materials that have band gap energies smaller than the illumination laser energy can improve the photothermal conversion efficiency owing to the presence of an additional light absorption channel.
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Cites
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Lee, S. E., Liu, G. L., Kim, F., & Lee, L. P. (2009) · Nano Letters · doi:10.1021/nl802689k · Cited by 224
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Metal/Semiconductor Hybrid Nanostructures for Plasmon‐Enhanced Applications
Jiang, R., Li, B., Fang, C., & Wang, J. (2014) · Advanced Materials · doi:10.1002/adma.201400203 · Cited by 1,156
Self-citationRecent Progress in Cancer Thermal Therapy Using Gold Nanoparticles
Abadeer, N. S., & Murphy, C. J. (2016) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.5b11232 · Cited by 919
Zhu, L., Gao, M., Peh, C. K. N., & Ho, G. W. (2018) · Materials Horizons · doi:10.1039/c7mh01064h · Cited by 733
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Sharma, A., Goyal, A. K., & Rath, G. (2018) · Journal of Drug Targeting · doi:10.1080/1061186x.2017.1400553 · Cited by 341
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de Melo‐Diogo, D., Pais‐Silva, C., Dias, D. R., Moreira, A. F., & Correia, I. J. (2017) · Advanced Healthcare Materials · doi:10.1002/adhm.201700073 · Cited by 267
Metadata
- Authors
- Chen, H., Shao, L., Ming, T., Sun, Z., Zhao, C., Yang, B., & Wang, J.
- Venue
- Small
- Publisher
- Wiley
- Published
- 2010-09-08
- Volume
- 6
- Issue
- 20
- Pages
- 2272-2280
- ISSN
- 1613-6810 (ISSN-L)
- 1613-6829
- OpenAlex
- W2036890691
- Cited by
- 634
- References
- 2
- FWCI
- 5.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, H., Shao, L., Ming, T., Sun, Z., Zhao, C., Yang, B., & Wang, J. (2010). Understanding the Photothermal Conversion Efficiency of Gold Nanocrystals. Small. https://doi.org/10.1002/smll.201001109
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