The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Cr‐Dopant Induced Breaking of Scaling Relations in CoFe Layered Double Hydroxides for Improvement of Oxygen Evolution Reaction
Abstract
Monodentate adsorption of oxygen intermediates results in a theoretical overpotential limit of ≈0.35 V for oxygen evolution reaction (OER), which causes the sluggish kinetics of the OER process. In this work, nonprecious chromium dopant is introduced into the self‐supported CoFe layered double hydroxides (LDHs) on nickel foam (Cr‐CoFe LDHs/NF) via a facile one‐step hydrothermal method, which exhibits a preeminent electrocatalytic activity toward the OER with an ultralow overpotential of 238 mV to obtain 10 mA cm−2 and a high stability after cyclic voltammetry for 5000 cycles in alkaline solution (1 m KOH). Density functional theory (DFT) calculations unveil that Cr dopants as new active sites could improve the electron‐donation ability of the resultant Cr‐CoFe LDHs due to the smaller electronegativity of Cr in comparison with Fe and Co. Therefore, the scaling relation of adsorption energy among four oxygen intermediates is broken and consequently the OER performance is further promoted. This work provides a strategy to develop efficient metal layered double hydroxide OER catalysts.
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Cites
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
Man, I. C., Su, H., Calle‐Vallejo, F., Hansen, H. A., Martínez, J. I., Inoglu, N. G., Kitchin, J., Jaramillo, T. F., Nørskov, J. K., & Rossmeisl, J. (2011) · ChemCatChem · doi:10.1002/cctc.201000397 · Cited by 4,769
Hydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Abild-Pedersen, F., Greeley, J., Studt, F., Rossmeisl, J., Munter, T. R., Moses, P. G., Skúlason, E., Bligaard, T., & Nørskov, J. K. (2007) · Physical Review Letters · doi:10.1103/physrevlett.99.016105 · Cited by 1,678
Chen, Z., Song, Y., Cai, J., Zheng, X., Han, D., Wu, Y., Zang, Y., Niu, S., Liu, Y., Zhu, J., et al. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201801834 · Cited by 1,075
Cited by
Zhang, H., Lv, Y., Chen, C., Lv, C., Wu, X., Guo, J., & Jia, D. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2021.120611 · Cited by 93
Metadata
- Authors
- Wen, L., Zhang, X., Liu, J., Li, X., Xing, C., Lyu, X., Cai, W., Wang, W., & Li, Y.
- Venue
- Small
- Publisher
- Wiley
- Published
- 2019-07-15
- Volume
- 15
- Issue
- 35
- Pages
- e1902373-e1902373
- ISSN
- 1613-6810 (ISSN-L)
- 1613-6829
- OpenAlex
- W2961014471
- Cited by
- 188
- References
- 5
- FWCI
- 4.28
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wen, L., Zhang, X., Liu, J., Li, X., Xing, C., Lyu, X., Cai, W., Wang, W., & Li, Y. (2019). Cr‐Dopant Induced Breaking of Scaling Relations in CoFe Layered Double Hydroxides for Improvement of Oxygen Evolution Reaction. Small. https://doi.org/10.1002/smll.201902373
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