The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Single or Double: Which Is the Altar of Atomic Catalysts for Nitrogen Reduction Reaction?
Abstract
Converting N 2 to NH 3 is an extremely valuable process but a long‐standing challenge in chemistry. The crux is the choice of catalysts, where single atomic catalysts (SAC) are always pursued as the altar of atomic catalysts. In this paper, double atomic catalysts (DAC) of TM 2‐C 2 N with SAC of TM‐C 2 N (TM = Cr, Mn, Fe, Co, and Ni) for nitrogen reduction reaction (NRR) are systematically compared. Unexpectedly, TM 2‐C 2 N are more suitable than TM‐C 2 N as catalysts for NRR. Moreover, the Mn 2‐C 2 N endows the highest catalytic activity with the lowest potential of −0.23 V versus RHE, which is the best among all reported calculation results for NRR under ambient conditions. As a result, a new way to design catalysts with DAC is provided.
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Cites
Effect of valence electron concentration on stability of fcc or bcc phase in high entropy alloys
Guo, S., Ng, C., Lu, J., & Liu, C. T. (2011) · Journal of Applied Physics · doi:10.1063/1.3587228 · Cited by 2,911
An efficient and pH-universal ruthenium-based catalyst for the hydrogen evolution reaction
Mahmood, J., Li, F., Jung, S.-M., Okyay, M. S., Ahmad, I., Kim, S.-J., Park, N., Jeong, H. Y., & Baek, J.-B. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2016.304 · Cited by 1,685
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Cited by
Guo, X., Gu, J., Lin, S., Zhang, S., Chen, Z., & Huang, S. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b13349 · Cited by 1,151
Self-citationDefect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
Ren, Y., Yu, C., Tan, X., Huang, H., Wei, Q., & Qiu, J. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03596c · Cited by 565
Breaking scaling relations for efficient CO2 electrochemical reduction through dual-atom catalysts
Ouyang, Y., Shi, L., Bai, X., Li, Q., & Wang, J. (2020) · Chemical Science · doi:10.1039/c9sc05236d · Cited by 382
Lv, X., Wei, W., Huang, B., Dai, Y., & Frauenheim, T. (2021) · Nano Letters · doi:10.1021/acs.nanolett.0c05080 · Cited by 369
Metadata
- Authors
- Chen, Z. W., Yan, J., & Jiang, Q.
- Venue
- Small Methods
- Publisher
- Wiley
- Published
- 2018-10-04
- Volume
- 3
- Issue
- 6
- ISSN
- 2366-9608 (ISSN-L)
- OpenAlex
- W2894988700
- Cited by
- 290
- References
- 3
- FWCI
- 7.47
- Type
- journal article
- Language
- en
- Open access
- closed
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