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Mechanism of Formation of Monodispersed Colloids by Aggregation of Nanosize Precursors
Open accessAbstract
It has been experimentally established in numerous cases that precipitation of monodispersed colloids from homogeneous solutions is a complex process. Specifically, it was found that in many systems nuclei, produced rapidly in a supersaturated solution, grow to nanosize primary particles (singlets), which then coagulate to form much larger final colloids in a process dominated by irreversible capture of these singlets. This paper describes a kinetic model that explains the formation of dispersions of narrow size distribution in such systems. Numerical simulations of the kinetic equations, with experimental model parameter values, are reported. The model was tested for a system involving formation of uniform spherical gold particles by reduction of auric chloride in aqueous solutions. The calculated average size, the width of the particle size distribution, and the time scale of the process agreed reasonably well with the experimental values. Copyright 1999 Academic Press.
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Cites
Theory, Production and Mechanism of Formation of Monodispersed Hydrosols
LaMer, V. K., & Dinegar, R. H. (1950) · Journal of the American Chemical Society · doi:10.1021/ja01167a001 · Cited by 3,894
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Formation mechanism and morphology in precipitation of vaterite—nano-aggregation or crystal growth?
Andreassen, J.-P. (2005) · Journal of Crystal Growth · doi:10.1016/j.jcrysgro.2004.09.090 · Cited by 212
Spherulitic Growth of Calcium Carbonate
Beck, R., & Andreassen, J.-P. (2010) · Crystal Growth & Design · doi:10.1021/cg901460g · Cited by 134
Direct Observation of Interactions between Nanoparticles and Nanoparticle Self-Assembly in Solution
Tan, S. F., Chee, S. W., Lin, G., & Mirsaidov, U. (2017) · Accounts of Chemical Research · doi:10.1021/acs.accounts.7b00063 · Cited by 133
Nanoscale magnetite: New synthesis approach, structure and properties
Novoselova, L. Y. (2021) · Applied Surface Science · doi:10.1016/j.apsusc.2020.148275 · Cited by 54
Metadata
- Authors
- Privman, V., Goia, D. V., Park, J., & Matijević, E.
- Venue
- Journal of Colloid and Interface Science
- Publisher
- Elsevier BV
- Published
- 1999-05
- Volume
- 213
- Issue
- 1
- Pages
- 36-45
- ISSN
- 0021-9797 (ISSN-L)
- OpenAlex
- W2109334065
- Cited by
- 386
- References
- 1
- FWCI
- 7.43
- Type
- journal article
- Language
- en
- Open access
- green
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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