Functionally graded optimisation of adsorption systems with phase change materials
Open accessAbstract
Adsorption phenomena are encountered in several engineering applications. One of its uses is in the storage and transport of gas in the form of adsorption tanks. The exothermic nature of the adsorption process decreases adsorption capacity presenting an impetus to understand the thermal characteristics of the gas storage process. Studies using mixtures of phase change materials and adsorbents in adsorption tanks demonstrate potential improvements in the adsorption capacity of the tanks. They also show that the distribution of phase change materials and adsorbent are important. Thus, this work presents two approaches for optimising the adsorbent domain. The first is to use a semi-analytic model to determine the best homogeneous material concentration for the adsorbent and phase change material for the vessel composition. The other is to use a 2D axisymmetric model to perform FGM optimisation to distribute material in the tank. Results for both models are presented and discussed for different conditions. The study shows that, for the cylindrical geometry, FGM optimisation is always, at least, marginally better than the homogeneous distribution from the semi-analytic model. However, FGM optimisation demands more computing time increases the complexity of implementation and results assembling. The semi-analytic approach is a possible alternative for optimising adsorption systems with phase change material mixed with adsorbents.
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Application of topology optimization to adsorption systems specifically is scarce.
“Its application to adsorption systems specifically, however, is quite scarce.”
From Topology optimisation of adsorption beds for cost-effective direct air capture (2026) · cites this paper as [24]
The Introduction (page not available) describes topology optimisation across several heat-transfer applications but names only one prior application to an adsorption system. This is consistent with limited use in adsorption, although the paper does not explicitly say that such applications are scarce. (LLM, conf=0.72)
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Cited by
Sorted by citations
Topology optimisation of adsorption beds for cost-effective direct air capture
Mallon, C., Thornton, A., Hill, M., Badia, S., & Grutering, N. (2026) · arXiv · doi:10.48550/arxiv.2609.14214
“In [23] and [24], optimizations considering adsorption in natural gas storage systems are conducted.”
- Authors
- Prado, D. S., Amigo, R. C. R., Hewson, R. W., & Silva, E. C. N.
- Affiliations
- Universidade de São Paulo (BR)
- Imperial College London (GB)
- Corresponding author
- Prado, D. S.
- Amigo, R. C. R.
- Hewson, R. W.
- Silva, E. C. N.
- Venue
- Structural and Multidisciplinary Optimization
- Published
- 2021-05-20
- Volume
- 64
- Issue
- 2
- Pages
- 473-503
- ISSN
- 1615-147X (ISSN-L)
- 1615-1488
- OpenAlex
- W3164874804
- Cited by
- 7
- References
- 0
- Citations by year
- 2026: 5 · 2022: 2
- FWCI
- 0.26
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Locations
- Structural and Multidisciplinary Optimization (publishedVersion, cc-by)
- Spiral (Imperial College London) (submittedVersion, cc-by)
- Funders
- Research Centre for Gas Innovation (2014/50279-4)
- Fundação de Amparo à Pesquisa do Estado de São Paulo (2014/, 2014 / 50279-4, 14/50279-4)
- Coordenação de Aperfeiçoamento de Pessoal de Nível Superior (2014/50279–4, 2018-1)
- Conselho Nacional de Desenvolvimento Científico e Tecnológico (302658/2018-1, 2014/50279-4, 2018-1)
- Universidade de São Paulo
- Topics
- Physical Sciences › Engineering › Civil and Structural Engineering › Topology Optimization in Engineering
- Physical Sciences › Engineering › Mechanics of Materials › Composite Structure Analysis and Optimization
- Physical Sciences › Engineering › Mechanical Engineering › Phase Change Materials Research
- Keywords
- functionally graded materials, phase change materials, gas storage, adsorption capacity, semi-analytical model, axisymmetric model, cylindrical geometry
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