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The importance of the lithium ion transference number in lithium/polymer cells
Open accessAbstract
Abstract Simulation results are presented for a lithium negative electrode, solid polymer separator, manganese dioxide composite positive electrode cell. In particular, we assess the effect of conductivity and transference number on cell performance, establishing criteria for situations when a trade-off between these two properties is expected. We show that polymer-electrolyte systems with a unity transference number have improved performance over systems with t0+ = 0.2, even when the conductivity is decreased by an order of magnitude. The improvements are primarily at higher rates of discharge, where the latter cell would be depleted of electrolyte due to large concentration gradients that develop. Cells with a unity transference number have larger energy densities and can attain higher peak-power densities.
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Citations
Cites
Modeling of Galvanostatic Charge and Discharge of the Lithium/Polymer/Insertion Cell
Doyle, M., Fuller, T. F., & Newman, J. (1993) · Journal of The Electrochemical Society · doi:10.1149/1.2221597 · Cited by 4,328
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Cited by
Promising Routes to a High Li+ Transference Number Electrolyte for Lithium Ion Batteries
Diederichsen, K. M., McShane, E. J., & McCloskey, B. D. (2017) · ACS Energy Letters · doi:10.1021/acsenergylett.7b00792 · Cited by 874
Perspectives for Polymer Electrolytes: A View from Fundamentals of Ionic Conductivity
Bocharova, V., & Sokolov, A. P. (2020) · Macromolecules · doi:10.1021/acs.macromol.9b02742 · Cited by 499
Fong, K. D., Self, J., Diederichsen, K. M., Wood, B. M., McCloskey, B. D., & Persson, K. A. (2019) · ACS Central Science · doi:10.1021/acscentsci.9b00406 · Cited by 239
Guo, R., & Han, W. (2022) · Materials Today Sustainability · doi:10.1016/j.mtsust.2022.100187 · Cited by 32
Metadata
- Authors
- Doyle, M., Fuller, T. F., & Newman, J.
- Venue
- Electrochimica Acta
- Publisher
- Elsevier BV
- Published
- 1994-09
- Volume
- 39
- Issue
- 13
- Pages
- 2073-2081
- ISSN
- 0013-4686 (ISSN-L)
- OpenAlex
- W2015745064
- Cited by
- 553
- References
- 1
- FWCI
- 5.37
- Type
- journal article
- Language
- en
- Open access
- green
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- Doyle, M., Fuller, T. F., & Newman, J. (1994). The importance of the lithium ion transference number in lithium/polymer cells. Electrochimica Acta. https://doi.org/10.1016/0013-4686(94)85091-7
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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