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Peroxymonosulfate enhanced visible light photocatalytic degradation bisphenol A by single-atom dispersed Ag mesoporous g-C3N4 hybrid
Open accessAbstract
Abstract Single-atom dispersed Ag modified mesoporous graphitic carbon nitride (Ag/mpg-C3N4) hybrid was synthesized by co-condensation method and employed as a visible light photocatalyst. In the presence of peroxymonosulfate (PMS), Ag/mpg-C3N4 showed excellent performance for the degradation of bisphenol A (BPA). 100% BPA and 80% TOC could be removed with 0.1 g/L catalyst and 1 mM PMS under visible light (λ > 400 nm) within 60 min. The reason for the enhanced performance is possibly due to the synergistic effect of single-atom Ag and mpg-C3N4. On the one hand, more visible light could be captured with the introduction of Ag; on the other hand, the existence of PMS promotes the separation efficiency of photogenerated electron-hole pairs. Electron spin resonance (ESR) and free radicals quenching experiment suggest that the major reactive oxygen species (ROS) are sulfate radical (SO4 −), superoxide radicals (O2 −) and photogenerated holes, while the role of hydroxyl radicals ( OH) is insignificant in this process. The findings of this work highlighted the great potential of g-C3N4 as photocatalysts and elucidated a new opportunity for PMS remediation of contaminated water.
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Buxton, G. V., Greenstock, C. L., Helman, W. P., & Ross, A. B. (1988) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555805 · Cited by 12,332
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
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Wang, L., Lan, X., Peng, W., & Wang, Z. (2021) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2020.124436 · Cited by 689
Guo, S., Wang, H., Yang, W., Fida, H., You, L., & Zhou, K. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.118250 · Cited by 499
Chen, F., Huang, G.-X., Yao, F.-B., Yang, Q., Zheng, Y.-M., Zhao, Q.-B., & Yu, H.-Q. (2020) · Water Research · doi:10.1016/j.watres.2020.115559 · Cited by 459
Sandwich-like Co3O4/MXene composite with enhanced catalytic performance for Bisphenol A degradation
Liu, Y., Luo, R., Li, Y., Qi, J., Wang, C., Li, J., Sun, X., & Wang, L. (2018) · Chemical Engineering Journal · doi:10.1016/j.cej.2018.04.155 · Cited by 282
Metadata
- Authors
- Wang, Y., Zhao, X., Cao, D., Wang, Y., & Zhu, Y.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2017-08
- Volume
- 211
- Pages
- 79-88
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2604236473
- Cited by
- 610
- References
- 2
- FWCI
- 31.23
- Type
- journal article
- Language
- en
- Open access
- green
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- Wang, Y., Zhao, X., Cao, D., Wang, Y., & Zhu, Y. (2017). Peroxymonosulfate enhanced visible light photocatalytic degradation bisphenol A by single-atom dispersed Ag mesoporous g-C3N4 hybrid. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2017.03.079
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