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P-doped ZnxCd1−xS solid solutions as photocatalysts for hydrogen evolution from water splitting coupled with photocatalytic oxidation of 5-hydroxymethylfurfural
Abstract
Abstract Photocatalytic water splitting over semiconductors without using of any electron sacrificial agents is essential to the conversion of solar energy into chemical energy. Herein, we report remarkable photocatalytic hydrogen production from pure water without the assistance of electron sacrificial agents by using P-doped ZnxCd1−xS with rich S vacancies (ZnxCd1−xS-P) as the photocatalyst. It is found that interstitial P doping in ZnxCd1−xS solid solutions with rich S vacancies can prolong the lifetime of charge carriers and enhance the generation and separation of photogenerated electrons-holes, resulting in a H2 evolution rate of up to 419 μmol h−1 g−1, which is 72 and 7.5 times higher than those of ZnS-P (5.8 μmol h−1 g−1) and CdS-P (56 μmol h−1 g−1), respectively. Furthermore, the introduction of biomass-derived compound 5-hydroxymethylfurfural (HMF) into this system further promotes the photocatalytic hydorgen evolution reaction and simultaneously obtains value-added HMF oxidation products.
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Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Wang, Q., Hisatomi, T., Jia, Q., Tokudome, H., Zhong, M., Wang, C., Pan, Z., Takata, T., Nakabayashi, M., Shibata, N., et al. (2016) · Nature Materials · doi:10.1038/nmat4589 · Cited by 1,684
Cited by
Kampouri, S., & Stylianou, K. C. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b00332 · Cited by 298
Li, S., Wang, L., Li, Y., Zhang, L., Wang, A., Xiao, N., Gao, Y., Li, N., Song, W., Ge, L., et al. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.05.001 · Cited by 298
Photocatalytic conversion of lignocellulosic biomass to valuable products
Liu, X., Duan, X., Wei, W., Wang, S., & Ni, B.-J. (2019) · Green Chemistry · doi:10.1039/c9gc01728c · Cited by 268
Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges
Pan, H., Li, J., Wang, Y., Xia, Q., Qiu, L., & Zhou, B. (2024) · Advanced Science · doi:10.1002/advs.202402651 · Cited by 67
Metadata
- Authors
- Ye, H.-F., Shi, R., Yang, X., Fu, W.-F., & Chen, Y.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2018-10
- Volume
- 233
- Pages
- 70-79
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2789725710
- Cited by
- 289
- References
- 2
- FWCI
- 6.11
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ye, H.-F., Shi, R., Yang, X., Fu, W.-F., & Chen, Y. (2018). P-doped ZnxCd1−xS solid solutions as photocatalysts for hydrogen evolution from water splitting coupled with photocatalytic oxidation of 5-hydroxymethylfurfural. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2018.03.060
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