The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Facile synthesis of single-nickel-atomic dispersed N-doped carbon framework for efficient electrochemical CO2 reduction
Abstract
Abstract While converting carbon dioxide (CO2) into value-added carbon products by electrolyzing offers a promising approach to mitigate global warming and store energy, poor selectivity and stability of catalysts still impede this conversion. Single-atom catalyst exhibits exceptional selectivity for CO2 electroreduction reaction in response to inhibiting hydrogen evolution reaction (HER), which is the major obstacle to the development of CO2 reduction. Herein we introduce a facile approach to obtain Ni-Nx sites encapsulating into carbon nanotubes with a nickel loading as high as 6.63 wt%. This catalyst exhibits high Faradaic efficiency approximately 95% for CO2 electroreduction to carbon monoxide (CO) in the wide potential range from −0.7 to −1.0 V, and the current density reaches 57.1 mA cm−2 at −1.0 V versus a reversible hydrogen electrode (RHE). Experiments and characterization results demonstrate that nickel chemical state and content play a vital role for CO2 electrocatalytic performance. Moreover, the simplifying of the synthesis may shed a new light on design single atom catalysts of electrochemistry in addition to CO2 reduction.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Liu, M., Pang, Y., Zhang, B., De Luna, P., Voznyy, O., Xu, J., Zheng, X., Dinh, C. T., Fan, F., Cao, C., et al. (2016) · Nature · doi:10.1038/nature19060 · Cited by 2,000
Li, C. W., & Kanan, M. W. (2012) · Journal of the American Chemical Society · doi:10.1021/ja3010978 · Cited by 2,000
Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Recent Advances in Inorganic Heterogeneous Electrocatalysts for Reduction of Carbon Dioxide
Zhu, D. D., Liu, J. L., & Qiao, S. Z. (2016) · Advanced Materials · doi:10.1002/adma.201504766 · Cited by 1,594
Cited by
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Metal‐Nitrogen‐Doped Carbon Materials as Highly Efficient Catalysts: Progress and Rational Design
Shi, Z., Yang, W., Gu, Y., Liao, T., & Sun, Z. (2020) · Advanced Science · doi:10.1002/advs.202001069 · Cited by 470
Wang, Y., Liu, Y., Liu, W., Wu, J., Li, Q., Feng, Q., Chen, Z., Xiong, X., Wang, D., & Lei, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02833a · Cited by 303
Metadata
- Authors
- Lu, P., Yang, Y., Yao, J., Wang, M., Dipazir, S., Yuan, M., Zhang, J., Wang, X., Xie, Z., & Zhang, G.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2019-02
- Volume
- 241
- Pages
- 113-119
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2891046017
- Cited by
- 287
- References
- 5
- FWCI
- 8.54
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lu, P., Yang, Y., Yao, J., Wang, M., Dipazir, S., Yuan, M., Zhang, J., Wang, X., Xie, Z., & Zhang, G. (2019). Facile synthesis of single-nickel-atomic dispersed N-doped carbon framework for efficient electrochemical CO2 reduction. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2018.09.025
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