The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Holey graphitic carbon nitride (g-CN) supported bifunctional single atom electrocatalysts for highly efficient overall water splitting
Abstract
Abstract Downsizing metal-based catalysts to construct single atom catalysts (SACs) is currently an emerging focus in research community of electrocatalysis, however, encountering the common aggregation of metal sites. Herein, the catalytic performance of holey g-CN supported SACs (Ti, V, Cr, Mn, Fe, Co and Ni) toward hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) are evaluated. Co1/g-CN and Ni1/g-CN are identified as the most efficient bifunctional single atom catalysts for overall water splitting, capable of driving HER/OER simultaneously with overpotentials being as low as 0.15/0.61 V and 0.12/0.40 V, outperforming the commercial Pt and IrO2. Remarkably, the d band centers of TM atoms can act as an efficient descriptor for the interaction strength between intermediates and TM/g-CN, which can be tuned to further optimize the catalytic activity. This work heralds a new family of bifunctional single atom electrocatalysts for overall water splitting, elucidating a useful guideline for designing advanced SACs.
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Cites
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
Man, I. C., Su, H., Calle‐Vallejo, F., Hansen, H. A., Martínez, J. I., Inoglu, N. G., Kitchin, J., Jaramillo, T. F., Nørskov, J. K., & Rossmeisl, J. (2011) · ChemCatChem · doi:10.1002/cctc.201000397 · Cited by 4,769
An efficient and pH-universal ruthenium-based catalyst for the hydrogen evolution reaction
Mahmood, J., Li, F., Jung, S.-M., Okyay, M. S., Ahmad, I., Kim, S.-J., Park, N., Jeong, H. Y., & Baek, J.-B. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2016.304 · Cited by 1,685
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Self-citationChen, Z., Song, Y., Cai, J., Zheng, X., Han, D., Wu, Y., Zang, Y., Niu, S., Liu, Y., Zhu, J., et al. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201801834 · Cited by 1,075
Photoelectrochemical water splitting in separate oxygen and hydrogen cells
Landman, A., Dotan, H., Shter, G. E., Wullenkord, M., Houaijia, A., Maljusch, A., Grader, G. S., & Rothschild, A. (2017) · Nature Materials · doi:10.1038/nmat4876 · Cited by 572
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Xie, C., Li, Y., Wang, Q., Sun, D., Tang, Y., & Wang, H. (2020) · Carbon Energy · doi:10.1002/cey2.67 · Cited by 401
Self-citationNon-carbon-supported single-atom site catalysts for electrocatalysis
Zheng, X., Li, P., Dou, S., Sun, W., Pan, H., Wang, D., & Li, Y. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00248a · Cited by 346
Li, J., Zhou, Y., Tang, W., Zheng, J., Gao, X., Wang, N., Chen, X., Wei, M., Xiao, X., & Chu, W. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119861 · Cited by 65
Xu, J., Li, R., Zeng, R., Yan, X., Zhao, Q., Ba, J., Luo, W., & Meng, D. (2020) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.0c09615 · Cited by 38
Metadata
- Authors
- Lv, X., Wei, W., Wang, H., Huang, B., & Dai, Y.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2020-05
- Volume
- 264
- Pages
- 118521
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2994628508
- Cited by
- 226
- References
- 5
- FWCI
- 4.33
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lv, X., Wei, W., Wang, H., Huang, B., & Dai, Y. (2020). Holey graphitic carbon nitride (g-CN) supported bifunctional single atom electrocatalysts for highly efficient overall water splitting. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2019.118521
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