Cited by 145Supercapacitor Materials and FabricationMXene and MAX Phase MaterialsElectrocatalysts for Energy Conversion

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Boron and nitrogen Co-doped holey graphene aerogels with rich B–N motifs for flexible supercapacitors

Zou, Xiaoxiao, Wu, Dapeng, Mu, Yifang, Xing, Luyang, Zhang, Wenchao, Gao, Zhiyong, Xu, Fang, Jiang, Kai·2020·Carbon

DOI 10.1016/j.carbon.2019.12.018

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Abstract

Abstract Boron and Nitrogen co-doped holey graphene aerogels (BN-HGA) are fabricated using ammonia borane as triple-functional precursor. The as-prepared BN-HGA possesses high specific surface area (249 m2 g−1) and rich B–N motifs with high surface polarity, which contributes to the rich and stable redox sites for the enhanced pseudo-capacitance. Moreover, the high hydrogen content in the ammonia borane cultures a reducing environment to preserve the integrity of carbon matrix, which gives rise to the high electronic conductivity. In addition, the well-developed hierarchically porous structure facilitates the ion diffusion in the electrode. Thanks to these structural merits, the BN-HGA electrode furnishes good specific capacitance of 456 F g−1 at 1 A g−1 in three-electrode systems using sulfuric acid as electrolyte. Meanwhile, the all-solid-state flexible supercapacitors based on the symmetric BN-HGA electrodes demonstrate high specific capacitance (345 mF cm −2 at 1 mA cm −2) and outstanding rate performance (80% retention at 20 mA cm −2). Furthermore, the flexible supercapacitor exhibits pleasant flexibility with marginable capacity loss as bent to arbitrary angles, which endows it a promising device for wearable energy storage.

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Authors: Zou, X., Wu, D., Mu, Y., Xing, L., Zhang, W., Gao, Z., Xu, F., & Jiang, K.
Affiliations: Henan Normal University (CN)
University of Wollongong (AU)
Corresponding author: Wu, Dapeng
Gao, Zhiyong
Jiang, Kai
ORCID: Wu, Dapeng
Zhang, Wenchao
Gao, Zhiyong
Xu, Fang
Jiang, Kai
Venue: Carbon
Publisher: Elsevier BV
Published: 2020-04
Volume: 159
Pages: 94-101
ISSN: 0008-6223 (ISSN-L)
DOI: 10.1016/j.carbon.2019.12.018
OpenAlex: W2995179902
Cited by: 145
References: 0
Citations by year: 2026: 19 · 2025: 18 · 2024: 19 · 2023: 20 · 2022: 24 · 2021: 34 · 2020: 11
FWCI: 5.35
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
www.elsevier.com/legal/tdmrep-license (tdm)
Locations: Carbon (publishedVersion)
Research Online (University of Wollongong) (submittedVersion)
Funders: National Natural Science Foundation of China
Topics: Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Keywords: flexible supercapacitors, all-solid-state supercapacitors, pseudocapacitance, specific capacitance, hierarchical porous structure, ion diffusion, rate capability, wearable energy storage

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Boron and nitrogen Co-doped holey graphene aerogels with rich B–N motifs for flexible supercapacitors

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