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Boron and nitrogen Co-doped holey graphene aerogels with rich B–N motifs for flexible supercapacitors
Abstract
Abstract Boron and Nitrogen co-doped holey graphene aerogels (BN-HGA) are fabricated using ammonia borane as triple-functional precursor. The as-prepared BN-HGA possesses high specific surface area (249 m2 g−1) and rich B–N motifs with high surface polarity, which contributes to the rich and stable redox sites for the enhanced pseudo-capacitance. Moreover, the high hydrogen content in the ammonia borane cultures a reducing environment to preserve the integrity of carbon matrix, which gives rise to the high electronic conductivity. In addition, the well-developed hierarchically porous structure facilitates the ion diffusion in the electrode. Thanks to these structural merits, the BN-HGA electrode furnishes good specific capacitance of 456 F g−1 at 1 A g−1 in three-electrode systems using sulfuric acid as electrolyte. Meanwhile, the all-solid-state flexible supercapacitors based on the symmetric BN-HGA electrodes demonstrate high specific capacitance (345 mF cm −2 at 1 mA cm −2) and outstanding rate performance (80% retention at 20 mA cm −2). Furthermore, the flexible supercapacitor exhibits pleasant flexibility with marginable capacity loss as bent to arbitrary angles, which endows it a promising device for wearable energy storage.
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“Additionally, the higher electronegativity of O, in comparison to C and N, may lead to the doped B forming a C−B−O bond.42”
From Iron–Cobalt Nanoparticles Embedded in B,N-Doped Chitosan-Derived Porous Carbon Aerogel for Overall Water Splitting (2024) · cites this paper as [42]
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Metadata
- Authors
- Zou, X., Wu, D., Mu, Y., Xing, L., Zhang, W., Gao, Z., Xu, F., & Jiang, K.
- Affiliations
- Henan Normal University (CN)
- University of Wollongong (AU)
- Corresponding author
- Wu, Dapeng
- Gao, Zhiyong
- Jiang, Kai
- Venue
- Carbon
- Publisher
- Elsevier BV
- Published
- 2020-04
- Volume
- 159
- Pages
- 94-101
- ISSN
- 0008-6223 (ISSN-L)
- OpenAlex
- W2995179902
- Cited by
- 145
- References
- 0
- Citations by year
- 2026: 19 · 2025: 18 · 2024: 19 · 2023: 20 · 2022: 24 · 2021: 34 · 2020: 11
- FWCI
- 5.35
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- www.elsevier.com/tdm/userlicense/1.0/ (tdm)
- www.elsevier.com/legal/tdmrep-license (tdm)
- Locations
- Carbon (publishedVersion)
- Research Online (University of Wollongong) (submittedVersion)
- Funders
- National Natural Science Foundation of China
- Topics
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Keywords
- flexible supercapacitors, all-solid-state supercapacitors, pseudocapacitance, specific capacitance, hierarchical porous structure, ion diffusion, rate capability, wearable energy storage
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