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Reticular chemistry in the rational synthesis of functional zirconium cluster-based MOFs
Open accessAbstract
Abstract In the past two decades, reticular chemistry has developed into a powerful tool for the design and synthesis of porous, crystalline framework materials. The discovery of the first hexanuclear, zirconium cluster-based MOF (i.e. UiO-66; fcu net) led to a vast library of functional Zr-MOFs with various properties. The versatile connectivity of zirconium hexanuclear clusters and the adaptable tunability of organic ligands have resulted in the rational synthesis of a large set of Zr-MOFs based on edge-transitive nets; these nets commonly exists in crystalline network structures as suggested by reticular chemistry. In this review, we summarize recent advances in the synthesis of zirconium cluster-based MOFs in the light of reticular chemistry design principles. Isoreticular tuning of MOF parent structures and post-synthetic modification of Zr-MOFs for targeted applications are also deliberated.
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Metadata
- Authors
- Chen, Z., Hanna, S. L., Redfern, L. R., Alezi, D., Islamoglu, T., & Farha, O. K.
- Venue
- Coordination Chemistry Reviews
- Publisher
- Elsevier BV
- Published
- 2019-05
- Volume
- 386
- Pages
- 32-49
- ISSN
- 0010-8545 (ISSN-L)
- OpenAlex
- W2914456976
- Cited by
- 495
- References
- 0
- FWCI
- 20.89
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Chen, Z., Hanna, S. L., Redfern, L. R., Alezi, D., Islamoglu, T., & Farha, O. K. (2019). Reticular chemistry in the rational synthesis of functional zirconium cluster-based MOFs. Coordination Chemistry Reviews. https://doi.org/10.1016/j.ccr.2019.01.017
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