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Ti3C2Tx MXene core-shell spheres for ultrahigh removal of mercuric ions

Open access
Shahzad, Asif, Nawaz, Mohsin, Moztahida, Mokrema, Jang, Jiseon, Tahir, Khurram, Kim, Jiho, Lim, Youngsu, Vassiliadis, Vassilios S., Woo, Seung Han, Lee, Dae Sung·2019·Chemical Engineering Journal

Abstract

Abstract Two-dimensional (2-D) titanium carbide MXene core (Ti3C2Tx) shell aerogel spheres (MX-SA) for mercuric ion removal were designed and fabricated with varying concentrations of Ti3C2Tx MXene and sodium alginate (SA) using a facile method. Owing to their unique inside structures, high porosities, large specific surface areas, oxygenated functional groups of MXene nanosheets, and available active binding sites, the synthesized microspheres constitute a unique adsorbent for heavy metals removal in water. The MX-SA4:20 spheres exhibit an exceptional adsorption capacity of 932.84 mg/g for Hg2+, which is among the highest value reported for adsorbents. The adsorbent exhibits high single- and multi-component removal efficiencies, with 100% efficiency for Hg2+ and >90% efficiency for five heavy metal ions. The synthesized materials are highly efficient for Hg2+ removal under extreme pH conditions (0.5–1.0 M HNO3) and have additional excellent reproducible properties. The micro-size and spherical shape of MX-SA4:20 also allow it to be used in column-packed devices.

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Metadata

Authors
Shahzad, A., Nawaz, M., Moztahida, M., Jang, J., Tahir, K., Kim, J., Lim, Y., Vassiliadis, V. S., Woo, S. H., & Lee, D. S.
Venue
Chemical Engineering Journal
Publisher
Elsevier BV
Published
2019-07
Volume
368
Pages
400-408
ISSN
1385-8947 (ISSN-L)
OpenAlex
W2915637182
Cited by
210
References
2
FWCI
9.07
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: Ti3C2Tx MXene core-shell spheres for ultrahigh removal of mercuric ions. https://app.cochat.ai/papers/10.1016/j.cej.2019.02.160
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Shahzad, A., Nawaz, M., Moztahida, M., Jang, J., Tahir, K., Kim, J., Lim, Y., Vassiliadis, V. S., Woo, S. H., & Lee, D. S. (2019). Ti3C2Tx MXene core-shell spheres for ultrahigh removal of mercuric ions. Chemical Engineering Journal. https://doi.org/10.1016/j.cej.2019.02.160

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