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Synthesis and Electrochemical Properties of Two-Dimensional RGO/Ti3C2Tx Nanocomposites
Open accessAbstract
MXene is a new type of two-dimensional layered material. Herein, a GO/Ti3C2Tx nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti3C2Tx was transformed into RGO/Ti3C2Tx under high temperature with Ar/H2. The prepared samples were characterized using X-ray diffraction (XRD), Raman measurement, scanning electron microscopy (SEM), energy disperse spectroscopy (EDS), and X-ray photoelectron spectroscopy (XPS). As an electrode material in lithium-ion batteries, the RGO/Ti3C2Tx nanocomposite exhibited an excellent electrochemical performance and an excellent rate performance. Compared to pure Ti3C2Tx, the nanocomposite had a better reversible capacity at different current densities and had no attenuation after 200 cycles, which is one time higher than pure Ti3C2Tx. The improvement in the specific capacity was due to the excellent electrical conductivity and the unique structure of RGO, in which a charge transfer bridge was built among the Ti3C2Tx flakes. Such a bridge shortened the transmission distance of the electrons and ions and effectively controlled the restacking of the laminated materials.
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MXene utilized in this study can be oxidized at temperature higher than 600 °C.
“the MXene utilized in this study can be oxidized at temperature higher than 600 °C [20, 32–34]”
From Hybrid MXene/reduced graphene oxide aerogel microspheres for hydrogen evolution reaction (2021) · cites this paper as [34]
The Introduction identifies the MXene as Ti3C2Tx, and Experimental Section 2.2 describes heating its composite at 450 °C in argon and hydrogen. Neither passage addresses oxidation above 600 °C; searches for that temperature and for thermal oxidation found no supporting passage in our copy. Page numbers were unavailable. (LLM, conf=0.75)
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“As a result, a large number of hydrogen bonds between the surface of modified CC and MXene make them tightly combine together and thus increase the stability of CMCM electrodes.(29) CV curves of CC, OPMCC, and CMCC in the sulfuric acid electrolyte are shown in Figure S1.”
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Harnessing the unique properties of MXenes for advanced rechargeable batteries
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“These peaks are attributed to the presence of oxygen-containing functional groups on the RGO in the In2O3/RGO NCs, as reported in previous studies [46,47].”
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Metadata
- Authors
- Shen, C., Wang, L., Zhou, A., Wang, B., Wang, X., Lian, W., Hu, Q., Qin, G., & Liu, X.
- Affiliations
- Henan Polytechnic University (CN)
- Chinese Academy of Sciences (CN)
- University of Manchester (GB)
- Corresponding author
- Wang, Libo
- Venue
- Nanomaterials
- Publisher
- MDPI AG
- Published
- 2018-01-31
- Volume
- 8
- Issue
- 2
- Pages
- 80
- ISSN
- 2079-4991 (ISSN-L)
- PMC
- PMC5853712
- OpenAlex
- W2785719750
- Cited by
- 152
- References
- 56
- Citations by year
- 2026: 15 · 2025: 9 · 2024: 19 · 2023: 35 · 2022: 25 · 2021: 12 · 2020: 21 · 2019: 15 · 2018: 1
- FWCI
- 4.57
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- Nanomaterials (publishedVersion, cc-by)
- Europe PMC (PubMed Central) (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Research Explorer (The University of Manchester) (submittedVersion, cc-by)
- Funders
- National Natural Science Foundation of China (51403056, 51472075, 134100510008, 51772077, T2013-4)
- Henan Polytechnic University (T2013‐4)
- Henan Province Science and Technology Innovation Talent Program
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Keywords
- MXene, Ti3C2Tx, reduced graphene oxide, lithium-ion battery anodes, electrochemical performance, rate capability, reversible capacity, two-dimensional layered materials
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