Bisphenol A degradation using waste antivirus copper film with enhanced sono-Fenton-like catalytic oxidation
Abstract
This study investigated the applicability of waste antivirus copper film (CF) as a Fenton-like catalyst. The reaction activity of H 2 O 2 and CF in combination was significantly enhanced by ultrasound (US) irradiation, and the synergy factor calculated from bisphenol A (BPA) degradation using CF-H 2 O 2-US was 9.64 compare to that of dual factors. Photoluminescence analyses were conducted to compare the generation of hydroxyl radicals during both processes. In this sono-Fenton-like process, BPA degradation was affected by solution pH, temperature, ultrasound power, CF size, H 2 O 2 dose, and initial BPA concentration. The BPA degradation curves showed an induction period (first stage) and a rapid degradation period (second stage). Process efficiency was totally and partially enhanced in the presence of chloride and carbonate ions, respectively. Chemical scavenger tests showed that both free and surface-bound hydroxyl radicals participate in BPA degradation under the sono-Fenton-like process using CF. The functional groups and copper crystals on the CF surface remained unchanged after five consecutive reuses, and the BPA degradation efficiency of CF was maintained over 80% during the reuse processes as a sono-Fenton-like catalyst.
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In the sono-Fenton reaction with copper film, carbonate ions inhibited the degradation; further addition of the ions increased the degradation but did not reach the control reaction.
“In the case of sono-Fenton reaction with copper film, the carbonate ions inhibited the degradation. Further addition of the ions increased the degradation but did not reach the control reaction [107].”
From Advanced Oxidation Processes for Degradation of Water Pollutants—Ambivalent Impact of Carbonate Species: A Review (2023) · cites this paper as [107]
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Rayaroth, M. P., Boczkaj, G., Aubry, O., Aravind, U. K., & Aravindakumar, C. T. (2023) · Water · doi:10.3390/w15081615 · Cited by 171 · see citing works
- Authors
- Chu, J.-H., Kang, J.-K., Park, S.-J., & Lee, C.-G.
- Affiliations
- Ajou University (KR)
- Seoul National University (KR)
- Hankyong National University (KR)
- Corresponding author
- Lee, Chang-Gu
- Venue
- Chemosphere
- Publisher
- Elsevier BV
- Published
- 2021-08
- Volume
- 276
- Pages
- 130218
- ISSN
- 0045-6535 (ISSN-L)
- OpenAlex
- W3138439470
- Cited by
- 47
- References
- 71
- Citations by year
- 2026: 3 · 2025: 6 · 2024: 9 · 2023: 13 · 2022: 8 · 2021: 8
- FWCI
- 2.83
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- Chemosphere (publishedVersion)
- PubMed (publishedVersion)
- Funders
- National Research Foundation of Korea (NRF-2018R1C1B5044937)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
- Physical Sciences › Materials Science › Materials Chemistry › Ultrasound and Cavitation Phenomena
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
- Keywords
- bisphenol A degradation, sonication, hydrogen peroxide, hydroxyl radicals, catalyst recycling, induction period, wastewater treatment
- MeSH terms
- Bisphenol A Compounds, Benzhydryl Compounds, Copper, Hydrogen Peroxide, Oxidation-Reduction, Phenols
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