Electrocatalytic oxidation of small organic molecules in acid medium: Enhancement of activity of noble metal nanoparticles and their alloys by supporting or modifying them with metal oxides
Open accessAbstract
Different approaches to enhancement of electrocatalytic activity of noble metal nanoparticles during oxidation of small organic molecules (namely potential fuels for low-temperature fuel cells such as methanol, ethanol and formic acid) are described. A physical approach to the increase of activity of catalytic nanoparticles (e.g. platinum or palladium) involves nanostructuring to obtain highly dispersed systems of high surface area. Recently, the feasibility of enhancing activity of noble metal systems through the formation of bimetallic (e.g. PtRu, PtSn, and PdAu) or even more complex (e.g. PtRuW, PtRuSn) alloys has been demonstrated. In addition to possible changes in the electronic properties of alloys, specific interactions between metals as well as chemical reactivity of the added components have been postulated. We address and emphasize here the possibility of utilization of noble metal and alloyed nanoparticles supported on robust but reactive high surface area metal oxides (e.g. WO 3, MoO 3, TiO 2, ZrO 2, V 2 O 5, and CeO 2) in oxidative electrocatalysis. This paper concerns the way in which certain inorganic oxides and oxo species can act effectively as supports for noble metal nanoparticles or their alloys during electrocatalytic oxidation of hydrogen and representative organic fuels. Among important issues are possible changes in the morphology and dispersion, as well as specific interactions leading to the improved chemisorptive and catalytic properties in addition to the feasibility of long time operation of the discussed systems.
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Carbon-supported Pt-alloy systems are known as solid solutions of Pt and other metal(s), among which carbon-supported Pt-based bimetallic alloys are popular electrocatalysts in PEMFCs.
“Carbon-supported Pt-alloy systems are known as solid solutions of Pt and other metal(s), among which carbonsupported Pt-based bimetallic alloys are popular electrocatalysts in PEMFCs.13,57,396,397”
From Carbon-Supported Pt-Based Alloy Electrocatalysts for the Oxygen Reduction Reaction in Polymer Electrolyte Membrane Fuel Cells: Particle Size, Shape, and Composition Manipulation and Their Impact to Activity (2015) · cites this paper as [397]
Section 4 says Pt and Ru can form a solid solution in a binary alloy, depending on their ratio; it does not say that Pt alloys generally are solid solutions. Sections 1 and 3 discuss Pt-based bimetallic electrocatalysts for fuel-cell reactions, but do not establish that carbon-supported Pt-based bimetallic alloys are popular in PEMFCs. Section 7 discusses a carbon-supported Pt–ceria material for PEMFCs, not a bimetallic alloy. (LLM, conf=0.86)
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Self-citation
Flagged first, then by citations
Research works printed but not linked: 1
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Cited by
Sorted by citations
Wang, Y.-J., Zhao, N., Fang, B., Li, H., Bi, X. T., & Wang, H. (2015) · Chemical Reviews · doi:10.1021/cr500519c · Cited by 1,267 · see citing works
- Authors
- Kulesza, P. J., Pieta, I. S., Rutkowska, I. A., Wadas, A., Marks, D., Klak, K., Stobinski, L., & Cox, J. A.
- Affiliations
- University of Warsaw (PL)
- Miami University (US)
- Corresponding author
- Cox, James A.
- Venue
- Electrochimica Acta
- Publisher
- Elsevier BV
- Published
- 2013-11
- Volume
- 110
- Pages
- 474-483
- ISSN
- 0013-4686 (ISSN-L)
- PMC
- PMC3891784
- OpenAlex
- W2036782576
- Cited by
- 109
- References
- 114
- Citations by year
- 2026: 2 · 2025: 6 · 2024: 2 · 2023: 10 · 2022: 4 · 2021: 7 · 2020: 13 · 2019: 6 · 2018: 12 · 2017: 10 · 2016: 13 · 2015: 12 · 2014: 11 · 2013: 1
- FWCI
- 4.48
- Type
- journal article
- Language
- en
- Open access
- green
- www.ncbi.nlm.nih.gov
- Locations
- Electrochimica Acta (publishedVersion)
- PubMed (publishedVersion)
- PubMed Central (acceptedVersion)
- Funders
- National Science Center, Poland
- U.S. National Institutes of Health (R15GM087662-01)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Keywords
- electrocatalytic oxidation, noble metal nanoparticles, bimetallic alloys, metal oxide supports, methanol oxidation, ethanol oxidation, formic acid oxidation, low-temperature fuel cells, platinum, palladium, PtRu alloy, PtSn alloy, Au-Pd alloys, nanostructuring, metal-support interaction, chemisorption, acid medium
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
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