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Nanocomposites of nickel selenide supported on cube-shaped lidless graphitic boxes as efficient counter electrodes for quasi-solid-state dye-sensitized solar cells
Abstract
Abstract To obtain an efficient electrocatalyst with high conductivity and hence excellent electrocatalytic performance, nanocomposites of nickel selenide supported on cube-shaped lidless graphitic boxes (Graphitic-boxes/NiSe) are prepared as the counter electrode (CE) of quasi-solid-state dye-sensitized solar cells (QSDSSCs). In view of the extraordinary three-dimensional electron transportation pathway and high specific surface area for the cube-shaped graphitic boxes, good catalytic ability of NiSe, and their synergetic effect, the Graphitic-boxes/NiSe nanocomposite exhibits excellent electrocatalytic activity towards the reduction of I 3 − . Furthermore, the Graphitic-boxes/NiSe nanocomposite shows impressive electrochemical stability against the iodine-based electrolyte compared with NiSe and Pt. The QSDSSC with the Graphitic-boxes/NiSe CE yields power conversion efficiency of 8.26%, which is superior to the graphitic boxes CE (2.01%) and the NiSe CE (7.45%) as well, and exhibits good long-term stability.
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“The peaks located at 278 and 518 cm− 1 can be assigned to LO phonon and Tg mode of Ni-Se bond, respectively [68,69].”
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Metadata
- Authors
- Feng, C., Jin, Z., Zhang, M., & Wang, Z.-S.
- Affiliations
- Fudan University (CN)
- Corresponding author
- Wang, Zhong-Sheng
- Venue
- Electrochimica Acta
- Publisher
- Elsevier BV
- Published
- 2018-08
- Volume
- 281
- Pages
- 237-245
- ISSN
- 0013-4686 (ISSN-L)
- OpenAlex
- W2807267555
- Cited by
- 16
- References
- 56
- Citations by year
- 2025: 1 · 2024: 2 · 2022: 3 · 2021: 4 · 2020: 1 · 2019: 5
- FWCI
- 0.58
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- www.elsevier.com/tdm/userlicense/1.0/ (tdm)
- www.elsevier.com/legal/tdmrep-license (tdm)
- Locations
- Electrochimica Acta (publishedVersion)
- Funders
- Fudan University
- Science and Technology Commission of Shanghai Municipality (168014342, 2011-iChEM)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › TiO2 Photocatalysis and Solar Cells
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
- Keywords
- nickel selenide, counter electrode, quasi-solid-state dye-sensitized solar cells, electrocatalysis, iodide reduction, electrochemical stability, nanocomposites, power conversion efficiency, long-term stability
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