Cited by 197Supercapacitor Materials and FabricationCarbon Dioxide Capture TechnologiesAdvanced Cellulose Research Studies

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Sustainable hierarchical porous carbon aerogel from cellulose for high-performance supercapacitor and CO2 capture

Zhuo, Hao, Hu, Yijie, Tong, Xing, Zhong, Linxin, Peng, Xinwen, Sun, Runcang·2016·Industrial Crops and Products

DOI 10.1016/j.indcrop.2016.04.041

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Abstract

Fabrication of cost-effective and eco-friendly hierarchical porous carbons from the most abundant and widely available biomass cellulose represents a critical and sustainable way to solve the crisis of fossil resources. In this work, a hierarchical porous carbon aerogel with desirable macropores, mesopores, and micropores was obtained via dissolving-gelling and subsequent carbonizing-activating process. The CO2 activated carbon aerogel had a high specific surface area of 1364m2/g and a high specific capacitance of 328Fg−1 (0.5Ag−1, 1.0M H2SO4) as well as an outstanding cycling stability with 96% of the capacitance retention after 5000 charge/discharge cycles. More importantly, for the first time, we demonstrated that the cellulose-derived hierarchical porous carbon aerogel showed a good CO2 adsorption capacity of 3.42mmol/g (at 1atm and 298K), which indicates the possibility of using this carbon aerogel for CO2 capture.

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Authors: Zhuo, H., Hu, Y., Tong, X., Zhong, L., Peng, X., & Sun, R.
Affiliations: State Key Laboratory of Pulp and Paper Engineering (CN)
Corresponding author: Zhong, Linxin
Peng, Xinwen
ORCID: Zhuo, Hao
Hu, Yijie
Tong, Xing
Zhong, Linxin
Peng, Xinwen
Venue: Industrial Crops and Products
Publisher: Elsevier BV
Published: 2016-09
Volume: 87
Pages: 229-235
ISSN: 0926-6690 (ISSN-L)
DOI: 10.1016/j.indcrop.2016.04.041
OpenAlex: W2344089845
Cited by: 196
References: 34
Citations by year: 2026: 8 · 2025: 14 · 2024: 21 · 2023: 22 · 2022: 26 · 2021: 25 · 2020: 19 · 2019: 24 · 2018: 22 · 2017: 11 · 2016: 4
FWCI: 6.39
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Industrial Crops and Products (publishedVersion)
Funders: National Natural Science Foundation of China (21506068)
State Key Laboratory of Pulp and Paper Engineering (2015ZD03, 2015QN05)
Pearl River S&T Nova Program of Guangzhou
Guangdong natural Science Foundation (2014A030310319)
Science and Technology Program of Guangzhou (201504010033)
Major State Basic Research Projects of China (973-2012CB215302)
Fundamental Research Funds for the Central Universities
Topics: Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Physical Sciences › Materials Science › Biomaterials › Advanced Cellulose Research Studies
Keywords: cellulose, biomass-derived carbon, supercapacitor electrodes, CO2 adsorption, CO2 capture, specific capacitance, cycling stability, carbonization and activation

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Sustainable hierarchical porous carbon aerogel from cellulose for high-performance supercapacitor and CO2 capture

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