Hydrothermal and mechanically generated hemp hurd nanofibers for sustainable barrier coatings/films
Open accessAbstract
Residual hemp (Cannabis sativa) hurd fibers obtained from hydrothermal, carbonate, and kraft treatments were the resources used to obtain lignocellulosic nanofibers (LCNF) by using an ultra-fine friction grinder. The morphological, crystallinity, and chemical characteristics of the nanocellulose films were carried out using SEM, XRD, EDX and ToF-SIMS. Water barrier properties of the same were measured in terms of water contact angle, water vapor permeability (WVP) and water absorption. The barrier properties were found to be dependent not only on the lignin content and lignin distribution, but also on the film density and porous structure. LCNF films and coatings showed much higher water contact angle (WCA) (80°-102°) than films produced from the bleached CNF. WVP was found to be more dependent on the density of films than lignin content. Overall, LCNF-based films and coatings derived from hemp hurd residual fibers can contribute to a circular economy and sustainability.
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Hydrothermal pulping, a chemical-free process, has shown promising results in extracting fibers from hemp hurds.
“Furthermore, hydrothermal pulping, a chemical-free process, has shown promising results in extracting fibers from hemp hurds (Naithani et al. 2020; Tyagi et al. 2021).”
From A critical review of industrial fiber hemp anatomy, agronomic practices, and valorization into sustainable bioproducts (2025) · cites this paper as Tyagi et al. 2021
The hemp hurds biomass can be converted into pulp fibers by traditional chemical and mechanical pulping processes; for example, kraft, carbonate, and soda processes have been successfully used to isolate hemp hurds fibers.
“The hemp hurds biomass can be converted into pulp fibers by traditional chemical and mechanical pulping processes. For example, kraft, carbonate, and soda processes have been successfully used to isolate hemp hurds fibers (Naithani et al. 2020; Tyagi et al. 2021; Gaynor et al. 2024).”
From A critical review of industrial fiber hemp anatomy, agronomic practices, and valorization into sustainable bioproducts (2025) · cites this paper as Tyagi et al. 2021
Cites
Cannabis sativa: The Plant of the Thousand and One Molecules
Andre, C. M., Hausman, J.-F., & Guerriero, G. (2016) · Frontiers in Plant Science · doi:10.3389/fpls.2016.00019 · Cited by 1,544 · see citing works
Innovating Generation of Nanocellulose from Industrial Hemp by Dual Asymmetric Centrifugation
Agate, S., Tyagi, P., Naithani, V., Lucia, L., & Pal, L. (2020) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.9b05992 · Cited by 51 · see citing works
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Tyagi, P., Gutierrez, J. N., Lucia, L. A., Hubbe, M. A., & Pal, L. (2022) · Cellulose · doi:10.1007/s10570-022-04583-w · Cited by 19 · see citing works
Self-citationBasak, M., Broadway, M., Lewis, J., Starkey, H., Bloomquist, M., Peszlen, I., Davis, J., Lucia, L. A., & Pal, L. (2025) · BioResources · doi:10.15376/biores.20.2.basak · Cited by 22 · see citing works
“Furthermore, hydrothermal pulping, a chemical-free process, has shown promising results in extracting fibers from hemp hurds (Naithani et al. 2020; Tyagi et al. 2021).”
InfluentialSelf-citation
- Authors
- Tyagi, P., Gutierrez, J. N., Nathani, V., Lucia, L. A., Rojas, O. J., Hubbe, M. A., & Pal, L.
- Affiliations
- North Carolina State University (US)
- University of British Columbia (CA)
- Corresponding author
- Pal, Lokendra
- ORCID
- Venue
- Industrial Crops and Products
- Publisher
- Elsevier BV
- Published
- 2021-09
- Volume
- 168
- Pages
- 113582
- ISSN
- 0926-6690 (ISSN-L)
- OpenAlex
- W3161377049
- Cited by
- 56
- References
- 2
- Citations by year
- 2026: 12 · 2025: 12 · 2024: 5 · 2023: 12 · 2022: 12 · 2021: 3
- FWCI
- 2.06
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- www.elsevier.com/tdm/userlicense/1.0/ (tdm)
- www.elsevier.com/legal/tdmrep-license (tdm)
- www.elsevier.com/open-access/userlicense/1.0/ (am, 248 d)
- doi.org/10.15223/policy-017 (stm-asf)
- doi.org/10.15223/policy-037 (stm-asf)
- doi.org/10.15223/policy-012 (stm-asf)
- doi.org/10.15223/policy-029 (stm-asf)
- doi.org/10.15223/policy-004 (stm-asf)
- Locations
- Industrial Crops and Products (acceptedVersion)
- Aaltodoc (Aalto University) (submittedVersion, cc-by-nc-nd)
- Funders
- National Science Foundation (ECCS-1542015)
- North Carolina State University
- Topics
- Physical Sciences › Materials Science › Biomaterials › Advanced Cellulose Research Studies
- Physical Sciences › Materials Science › Polymers and Plastics › Natural Fiber Reinforced Composites
- Physical Sciences › Materials Science › Biomaterials › Nanocomposite Films for Food Packaging
- Keywords
- hemp hurd, nanocellulose films, barrier coatings, water vapor permeability, water contact angle, lignin content, lignin distribution, hydrothermal treatment, circular economy, sustainable packaging
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