Cited by 300Heavy metals in environmentAdsorption and biosorption for pollutant removalEnvironmental and Analytical Chemistry Studies

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Competitive sorption and desorption of heavy metals by individual soil components

Covelo, E.F., Vega, F.A., Andrade, M.L.·2007·Journal of Hazardous Materials

DOI 10.1016/j.jhazmat.2006.09.018

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Abstract

Knowledge of sorption and desorption of heavy metals by individual soil components should be useful for modelling the behaviour of soils of arbitrary composition when contaminated by heavy metals, and for designing amendments increasing the fixation of heavy metals by soils polluted by these species. In this study the competitive sorption and desorption of Cd, Cr, Cu, Ni, Pb and Zn by humified organic matter, Fe and Mn oxides, kaolinite, vermiculite and mica were investigated. Due to the homogeneity of the sorbents, between-metal competition for binding sites led to their preferences for one or another metal being much more manifest than in the case of whole soils. On the basis of k(d100) values (distribution coefficients calculated in sorption-desorption experiments in which the initial sorption solution contained 100mgL(-1) of each metal), kaolinite and mica preferentially sorbed and retained chromium; vermiculite, copper and zinc; HOM, Fe oxide and Mn oxide, lead (HOM and Mn oxide also sorbed and retained considerable amounts of copper). Mica only retained sorbed chromium, Fe oxide sorbed cadmium and lead, and kaolinite did not retain sorbed copper. The sorbents retaining the greatest proportions of sorbed metals were vermiculite and Mn oxide, but the ratios of k(d100) values for retention and sorption suggest that cations were least reversibly bound by Mn oxide, and most reversibly by vermiculite.

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Authors: Covelo, E. F., Vega, F. A., & Andrade, M. L.
Affiliations: Universidade de Vigo (ES)
Corresponding author: Covelo, E.F.
ORCID: Vega, F.A.
Venue: Journal of Hazardous Materials
Publisher: Elsevier BV
Published: 2007-02
Volume: 140
Issue: 1-2
Pages: 308-315
ISSN: 0304-3894 (ISSN-L)
DOI: 10.1016/j.jhazmat.2006.09.018
OpenAlex: W2064118317
Cited by: 300
References: 42
Citations by year: 2026: 16 · 2025: 15 · 2024: 19 · 2023: 27 · 2022: 14 · 2021: 13 · 2020: 20 · 2019: 17 · 2018: 19 · 2017: 20 · 2016: 16 · 2015: 13 · 2014: 15 · 2013: 13 · 2012: 15
FWCI: 6.33
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
www.elsevier.com/legal/tdmrep-license (tdm)
Locations: Journal of Hazardous Materials (publishedVersion)
PubMed (publishedVersion)
Funders: Ministerio de Educación, Cultura y Deporte (REN 2002-0187)
Xunta de Galicia (PGIDTI03PXIC3001PN)
Topics: Physical Sciences › Environmental Science › Pollution › Heavy metals in environment
Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
Physical Sciences › Environmental Science › Water Science and Technology › Environmental and Analytical Chemistry Studies
Keywords: heavy metal adsorption, competitive adsorption, desorption, soil components, humified organic matter, iron oxide, manganese oxide, kaolinite, vermiculite, mica, cadmium, chromium, copper, nickel, lead, zinc, distribution coefficient, metal retention, sorption reversibility, soil contamination
MeSH terms: Adsorption, Aluminum Silicates, Binding, Competitive, Kaolin, Oxides, Soil, Manganese Compounds, Metals, Heavy

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Competitive sorption and desorption of heavy metals by individual soil components

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