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Use of clinoptilolite for the removal of nickel ions from water: Kinetics and thermodynamics

Argun, Mehmet Emin·2008·Journal of Hazardous Materials

DOI 10.1016/j.jhazmat.2007.05.008

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Abstract

This paper describes the removal of Ni(II) ions from aqueous solutions using clinoptilolite. The effect of clinoptilolite level, contact time, and pH were determined. Different isotherms were also obtained using concentrations of Ni(II) ions ranging from 0.1 to 100 mg L(-1). The ion-exchange process follows second-order reaction kinetics and follows the Langmuir isotherm. The paper discusses thermodynamic parameters, including changes in Gibbs free energy, entropy, and enthalpy, for the ion-exchange of Ni(II) on clinoptilolite, and revealed that the ion-exchange process was spontaneous and exothermic under natural conditions. The maximum removal efficiency obtained was 93.6% at pH 7 and with a 45 min contact time (for 25 mg L(-1) initial concentration and a 15 g L(-1) solid-to-liquid ratio).

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Authors: Argun, M. E.
Affiliations: Selçuk University (TR)
Corresponding author: Argun, Mehmet Emin
ORCID: Argun, Mehmet Emin
Venue: Journal of Hazardous Materials
Publisher: Elsevier BV
Published: 2008-02
Volume: 150
Issue: 3
Pages: 587-595
ISSN: 0304-3894 (ISSN-L)
DOI: 10.1016/j.jhazmat.2007.05.008
OpenAlex: W2088107882
Cited by: 224
References: 37
Citations by year: 2026: 6 · 2025: 10 · 2024: 12 · 2023: 17 · 2022: 12 · 2021: 7 · 2020: 11 · 2019: 14 · 2018: 15 · 2017: 6 · 2016: 19 · 2015: 15 · 2014: 12 · 2013: 17 · 2012: 16
FWCI: 7.58
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Journal of Hazardous Materials (publishedVersion)
PubMed (publishedVersion)
Funders: Selçuk Üniversitesi
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
Physical Sciences › Environmental Science › Waste Management and Disposal › Chemical Synthesis and Characterization
Physical Sciences › Materials Science › Metals and Alloys › Extraction and Separation Processes
Keywords: clinoptilolite, nickel removal, heavy metal adsorption, ion exchange kinetics, second-order kinetics, Langmuir isotherm, adsorption thermodynamics, Gibbs free energy, pH effect, contact time, zeolite adsorbents
MeSH terms: Adsorption, Ion Exchange, Kinetics, Nickel, Thermodynamics, Waste Disposal, Fluid, Water Pollutants, Chemical, Zeolites, Water Purification

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Use of clinoptilolite for the removal of nickel ions from water: Kinetics and thermodynamics

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