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Cited by 186Arsenic contamination and mitigationAdsorption and biosorption for pollutant removalEnvironmental remediation with nanomaterials

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Removal of arsenic from water using granular ferric hydroxide: Macroscopic and microscopic studies

Guan, Xiao-Hong, Wang, Jianmin, Chusuei, Charles C.·2008·Journal of Hazardous Materials
DOI 10.1016/j.jhazmat.2007.12.012
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Abstract

Removal of arsenate from water using granular ferric hydroxide (GFH) was investigated under different pH and As(V) loading conditions, using batch equilibrium adsorption, FTIR, and EXAFS methods. The arsenate adsorption envelopes on GFH exhibited broad adsorption maxima when the initial As(V) concentration was less than 500 mg/L at sorbent concentration of 10 g/L. As the initial As(V) concentration increased to 500, 1000 or 2000 mg/L for the same sorbent concentration, distinct adsorption maxima appeared and shifted to lower pH. Acidimetric-alkalimetric titration and arsenic adsorption isotherm data indicated that the surface of GFH is high heterogeneous. FTIR spectra revealed that complexes of two different structures, bidentate and monodentate, were formed upon the adsorption of arsenate on GFH, and bidentate complexes were only observed at pH values greater than 6. The EXAFS analyses confirmed that arsenate form bidentate binuclear complexes with GFH at pH 7.4 as evidenced by an average Fe-As(V) bond distance of 3.32 A.

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Metadata

Authors
Guan, X.-H., Wang, J., & Chusuei, C. C.
Affiliations
Missouri University of Science and Technology (US)
Corresponding author
Wang, Jianmin
ORCID
Venue
Journal of Hazardous Materials
Publisher
Elsevier BV
Published
2008-08
Volume
156
Issue
1-3
Pages
178-185
ISSN
0304-3894 (ISSN-L)
DOI
10.1016/j.jhazmat.2007.12.012
OpenAlex
W2043927988
Cited by
186
References
1
Citations by year
2026: 2 · 2025: 3 · 2024: 7 · 2023: 10 · 2022: 8 · 2021: 12 · 2020: 8 · 2019: 13 · 2018: 12 · 2017: 11 · 2016: 9 · 2015: 13 · 2014: 14 · 2013: 15 · 2012: 16
FWCI
7.99
Type
journal article
Language
en
Open access
closed
Licence
www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations
  • Journal of Hazardous Materials (publishedVersion)
  • PubMed (publishedVersion)
Funders
  • U.S. Environmental Protection Agency
  • University of Delaware
  • University of Missouri
Topics
  • Physical Sciences › Environmental Science › Environmental Chemistry › Arsenic contamination and mitigation
  • Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
  • Physical Sciences › Environmental Science › Environmental Engineering › Environmental remediation with nanomaterials
Keywords
arsenate removal, granular ferric hydroxide, adsorption isotherms, arsenic adsorption, pH effect, binuclear iron complexes, surface heterogeneity, water treatment, heavy metal removal
MeSH terms
Adsorption, Arsenic, Ferric Compounds, Microscopy, Electron, Scanning, Water Pollutants, Chemical, Spectroscopy, Fourier Transform Infrared

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