Variable diffusivity homogeneous surface diffusion model and analysis of merits and fallacies of simplified adsorption kinetics equations
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Adsorption and ion exchange phenomena are encountered in several separation processes, which in turn, are of vital importance across various industries. Although the literature on adsorption kinetics modeling is rich, the majority of the models employed are empirical, based on chemical reaction kinetics or oversimplified versions of diffusion models. In this paper, the fifteen most popular simplified adsorption kinetics equations are presented and discussed. A new versatile variable-diffusivity two-phase homogeneous diffusion model is presented and used to evaluate the analytical adsorption models. Aspects of ion exchange kinetics are also addressed.
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The PSO model was applied as a method for comparison; physical or mechanistic interpretation of the empirical model would provide erroneous insight.
“The PSO model was applied as a method for comparison; therefore, physical or mechanistic interpretation of the empirical model would provide erroneous insight [35,36].”
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Cited by
Sorted by citations
- Authors
- Inglezakis, V. J., Fyrillas, M. M., & Park, J.
- Affiliations
- Nazarbayev University (KZ)
- Frederick University (CY)
- University of Wisconsin–Madison (US)
- Corresponding author
- Inglezakis, V.J.
- Venue
- Journal of Hazardous Materials
- Publisher
- Elsevier BV
- Published
- 2019-04
- Volume
- 367
- Pages
- 224-245
- ISSN
- 0304-3894 (ISSN-L)
- OpenAlex
- W2905743291
- Cited by
- 133
- References
- 108
- Citations by year
- 2026: 8 · 2025: 15 · 2024: 18 · 2023: 23 · 2022: 13 · 2021: 18 · 2020: 25 · 2019: 10
- FWCI
- 0.79
- Type
- journal article
- Language
- en
- Open access
- Locations
- Journal of Hazardous Materials (publishedVersion)
- PubMed (publishedVersion)
- Strathprints: The University of Strathclyde institutional repository (University of Strathclyde) (submittedVersion)
- Funders
- ORAU project “Hyperstiochiometry Activity in Metal Nanoparticle Interaction (HYPERActiv)” (SOE2015009)
- Nazarbayev University
- HORIZON 2020 project “Nanoporous and Nanostructured Materials for Medical Applications (NanoMed)” (H2020-MSCA-RISE-2016)
- European Commission (734641)
- CRoNoS – IC408 COST Action
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Chemistry › Spectroscopy › Adsorption, diffusion, and thermodynamic properties of materials
- Physical Sciences › Engineering › Biomedical Engineering › Environmental remediation with nanomaterials
- Keywords
- adsorption kinetics, variable diffusivity, ion exchange kinetics, separation processes
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Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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