The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Hybrid Aqueous/Non-aqueous Electrolyte for Safe and High-Energy Li-Ion Batteries
Open accessAbstract
Summary Recent breakthroughs in aqueous electrolytes made highly safe 3.0 V class aqueous Li-ion batteries possible. However, the formed solid-electrolyte interphase therein still cannot effectively support the desired energy-dense anode and cathode materials. In this work, we report a new class of electrolytes, by hybridizing aqueous with non-aqueous solvents, that inherits the non-flammability and non-toxicity characteristics from aqueous and better electrochemical stability from non-aqueous systems. The secondary interphasial ingredient (alkylcarbonate) introduced by non-aqueous component helps to expand the electrochemical window of the hybridized electrolyte to 4.1 V, which supports the operation of a 3.2 V aqueous Li-ion battery based on Li 4 Ti 5 O 12 and LiNi 0.5 Mn 1.5 O 4 to deliver a high energy density of 165 Wh/kg for >1,000 cycles. The understanding of how a better interphase could be tailored by regulating the inner-Helmholtz interfacial structures of the hybridized electrolyte provides important guidelines for designing future electrolytes and interphases for new battery chemistries.
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Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Self-citation“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
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Cited by
Rechargeable Batteries for Grid Scale Energy Storage
Zhu, Z., Jiang, T., Ali, M., Meng, Y., Jin, Y., Cui, Y., & Chen, W. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00289 · Cited by 1,769
Safe and high-rate supercapacitors based on an “acetonitrile/water in salt” hybrid electrolyte
Dou, Q., Lei, S., Wang, D.-W., Zhang, Q., Xiao, D., Guo, H., Wang, A., Yang, H., Li, Y., Shi, S., et al. (2018) · Energy & Environmental Science · doi:10.1039/c8ee01040d · Cited by 435
Electrochemical Zinc Ion Capacitors: Fundamentals, Materials, and Systems
Yin, J., Zhang, W., Alhebshi, N. A., Salah, N., & Alshareef, H. N. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202100201 · Cited by 325
Chen, J., Vatamanu, J., Xing, L., Borodin, O., Chen, H., Guan, X., Liu, X., Xu, K., & Li, W. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902654 · Cited by 260
Self-citationLocalized Water‐In‐Salt Electrolyte for Aqueous Lithium‐Ion Batteries
Jaumaux, P., Yang, X., Zhang, B., Safaei, J., Tang, X., Zhou, D., Wang, C., & Wang, G. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202107389 · Cited by 205
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Metadata
- Authors
- Wang, F., Borodin, O., Ding, M. S., Gobet, M., Vatamanu, J., Fan, X., Gao, T., Eidson, N., Liang, Y., Sun, W., Greenbaum, S., Xu, K., & Wang, C.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2018-05
- Volume
- 2
- Issue
- 5
- Pages
- 927-937
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W2789332115
- Cited by
- 442
- References
- 3
- FWCI
- 16.09
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Wang, F., Borodin, O., Ding, M. S., Gobet, M., Vatamanu, J., Fan, X., Gao, T., Eidson, N., Liang, Y., Sun, W., Greenbaum, S., Xu, K., & Wang, C. (2018). Hybrid Aqueous/Non-aqueous Electrolyte for Safe and High-Energy Li-Ion Batteries. Joule. https://doi.org/10.1016/j.joule.2018.02.011
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