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Cited by 253

The DOI matches its Crossref record; 53 of the 53 references it cites were found in a registry or an index.

A Dynamic, Electrolyte-Blocking, and Single-Ion-Conductive Network for Stable Lithium-Metal Anodes

Open access
Yu, Zhiao, Mackanic, David G., Michaels, Wesley, Lee, Minah, Pei, Allen, Feng, Dawei, Zhang, Qiuhong, Tsao, Yuchi, Amanchukwu, Chibueze V., Yan, Xuzhou, Wang, Hansen, Chen, Shucheng, Liu, Kai, Kang, Jiheong, Qin, Jian, Cui, Yi, Bao, Zhenan·2019·Joule
DOI 10.1016/j.joule.2019.07.025
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Abstract

Summary Implementation of lithium (Li)-metal anodes requires developments to solve the heterogeneity and instability issues of naturally formed solid-electrolyte interphase (SEI). The artificial SEI, as an alternative, enables an ideal interface by regulating critical features such as fast ion transport, conformal protection, and parasitic reaction mitigation. Herein, for the first time, we integrate all of these desired properties into a single matrix, the dynamic single-ion-conductive network (DSN), as a multifunctional artificial SEI. The DSN incorporates the tetrahedral Al(OR)4− (R = soft fluorinated linker) centers as both dynamic bonding motifs and counter anions, endowing it with flowability and Li+ single-ion conductivity. Simultaneously, the fluorinated linkers provide chain mobility and electrolyte-blocking capability. A solution-processed DSN coating was found to simultaneously hinder electrolyte penetration, mitigate side reactions between Li and electrolyte, maintain low interfacial impedance, and allow homogenous Li deposition. With this coating, long cycle life and high Coulombic efficiency are achieved for Li-metal battery in a commercial carbonate electrolyte.

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Metadata

Authors
Yu, Z., Mackanic, D. G., Michaels, W., Lee, M., Pei, A., Feng, D., Zhang, Q., Tsao, Y., Amanchukwu, C. V., Yan, X., Wang, H., Chen, S., Liu, K., Kang, J., Qin, J., Cui, Y., & Bao, Z.
Venue
Joule
Publisher
Elsevier BV
Published
2019-11
Volume
3
Issue
11
Pages
2761-2776
ISSN
2542-4351 (ISSN-L)
DOI
10.1016/j.joule.2019.07.025
OpenAlex
W2970746067
Cited by
253
References
53
FWCI
11.98
Type
journal article
Language
en
Open access
bronze

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CoChat. (2026). Citation check: A Dynamic, Electrolyte-Blocking, and Single-Ion-Conductive Network for Stable Lithium-Metal Anodes. https://app.cochat.ai/papers/10.1016/j.joule.2019.07.025
The paper
Yu, Z., Mackanic, D. G., Michaels, W., Lee, M., Pei, A., Feng, D., Zhang, Q., Tsao, Y., Amanchukwu, C. V., Yan, X., Wang, H., Chen, S., Liu, K., Kang, J., Qin, J., Cui, Y., & Bao, Z. (2019). A Dynamic, Electrolyte-Blocking, and Single-Ion-Conductive Network for Stable Lithium-Metal Anodes. Joule. https://doi.org/10.1016/j.joule.2019.07.025

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.