The DOI matches its Crossref record; 34 of the 34 references it cites were found in a registry or an index.
A Liquid Electrolyte with De-Solvated Lithium Ions for Lithium-Metal Battery
Open accessAbstract
Summary Traditional liquid electrolytes used in rechargeable batteries, fuel cells, and electrochemical capacitors composed of solvents, anions, and solvents solvated cations (e.g., lithium ions, Li+), follow classic “cations with solvation” electrolyte configuration and can be defined as “cations solvated electrolytes.” In these electrolytes, the de-solvation processes of solvated cations only occur when the cations inserted-deposited on the electrodes’ surface. Here, different from traditional electrolytes, a new liquid electrolyte with de-solvated Li+ was discovered (“Li+ de-solvated electrolyte”), since it merely composed of inactive “frozen-like” solvent and crystal-like salt solute. Inspiringly, its electrochemical stability was remarkably improved (extended to 4.5 V for “Li+ de-solvated ether-based electrolyte”). Ultra-stable high-energy-density lithium-metal batteries (LiNi0.8Co0.1Mn0.1O2//Li) were achieved (half-cell: 140 mAh g−1 after 830 cycles; full-cell: 170 mAh g−1 after 200 cycles under twice excessed Li). It is also surprising that this does not present any cathode-electrolyte interface (CEI) layer on the cycled NCM-811 surface benefit from the “Li+ de-solvated electrolyte.”
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Cited by
Cao, Z., Zheng, X., Qu, Q., Huang, Y., & Zheng, H. (2021) · Advanced Materials · doi:10.1002/adma.202103178 · Cited by 336
Historical development and novel concepts on electrolytes for aqueous rechargeable batteries
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Metadata
- Authors
- Chang, Z., Qiao, Y., Deng, H., Yang, H., He, P., & Zhou, H.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2020-08
- Volume
- 4
- Issue
- 8
- Pages
- 1776-1789
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W3042633680
- Cited by
- 265
- References
- 34
- FWCI
- 11.82
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Chang, Z., Qiao, Y., Deng, H., Yang, H., He, P., & Zhou, H. (2020). A Liquid Electrolyte with De-Solvated Lithium Ions for Lithium-Metal Battery. Joule. https://doi.org/10.1016/j.joule.2020.06.011
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