The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Cascade CO2 electroreduction enables efficient carbonate-free production of ethylene
Open accessAbstract
Summary CO2 electroreduction provides a route to convert waste emissions into chemicals such as ethylene (C2H4). However, the direct transformation of CO2-to-C2H4 suffers from CO2 loss to carbonate, consuming up to 72% of energy input. A cascade approach—coupling a solid-oxide CO2-to-CO electrochemical cell (SOEC) with a CO-to-C2H4 membrane electrode assembly (MEA)—would eliminate CO2 loss to carbonate. However, this approach requires a CO-to-C2H4 MEA with energy efficiency well beyond demonstrations to date. Focusing on the MEA, we find that an N-tolyl substituted tetrahydro-bipyridine film improves the stabilization of key reaction intermediates, while an SSC ionomer enhances CO transport to the Cu surface, enabling a C2H4 faradaic efficiency of 65% at 150 mA cm−2 for 110 h. Demonstrating a cascade SOEC-MEA approach, we achieve CO2-to-C2H4 with a ~48% reduction in energy intensity compared with the direct route. We further reduce the energy intensity by coupling CO electroreduction (CORR) with glucose electrooxidation.
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Cites
What would it take for renewably powered electrosynthesis to displace petrochemical processes?
De Luna, P., Hahn, C., Higgins, D., Jaffer, S. A., Jaramillo, T. F., & Sargent, E. H. (2019) · Science · doi:10.1126/science.aav3506 · Cited by 3,052
Self-citationThe technological and economic prospects for CO2 utilization and removal
Hepburn, C., Adlen, E., Beddington, J., Carter, E. A., Fuss, S., Mac Dowell, N., Minx, J. C., Smith, P., & Williams, C. K. (2019) · Nature · doi:10.1038/s41586-019-1681-6 · Cited by 2,523 · cited 1×
“6% of the total anthropogenic emissions.(3)”
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Self-citationCO 2 electrolysis to multicarbon products at activities greater than 1 A cm −2
García de Arquer, F. P., Dinh, C.-T., Ozden, A., Wicks, J., McCallum, C., Kirmani, A. R., Nam, D.-H., Gabardo, C., Seifitokaldani, A., Wang, X., et al. (2020) · Science · doi:10.1126/science.aay4217 · Cited by 1,517
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Cited by
CO 2 electrolysis to multicarbon products in strong acid
Huang, J. E., Li, F., Ozden, A., Sedighian Rasouli, A., García de Arquer, F. P., Liu, S., Zhang, S., Luo, M., Wang, X., Lum, Y., et al. (2021) · Science · doi:10.1126/science.abg6582 · Cited by 1,359
Self-citationGu, J., Liu, S., Ni, W., Ren, W., Haussener, S., & Hu, X. (2022) · Nature Catalysis · doi:10.1038/s41929-022-00761-y · Cited by 846
Electrochemical CO2 reduction in membrane-electrode assemblies
Ge, L., Rabiee, H., Li, M., Subramanian, S., Zheng, Y., Lee, J. H., Burdyny, T., & Wang, H. (2022) · Chem · doi:10.1016/j.chempr.2021.12.002 · Cited by 336
Self-citationLopez, G., Keiner, D., Fasihi, M., Koiranen, T., & Breyer, C. (2023) · Energy & Environmental Science · doi:10.1039/d3ee00478c · Cited by 284
Bipolar membrane electrolyzers enable high single-pass CO2 electroreduction to multicarbon products
Xie, K., Miao, R. K., Ozden, A., Liu, S., Chen, Z., Dinh, C.-T., Huang, J. E., Xu, Q., Gabardo, C. M., Lee, G., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-31295-3 · Cited by 270
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Metadata
- Authors
- Ozden, A., Wang, Y., Li, F., Luo, M., Sisler, J., Thevenon, A., Rosas-Hernández, A., Burdyny, T., Lum, Y., Yadegari, H., Agapie, T., Peters, J. C., Sargent, E. H., & Sinton, D.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2021-03
- Volume
- 5
- Issue
- 3
- Pages
- 706-719
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W3132233222
- Cited by
- 338
- References
- 4
- FWCI
- 10.45
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Ozden, A., Wang, Y., Li, F., Luo, M., Sisler, J., Thevenon, A., Rosas-Hernández, A., Burdyny, T., Lum, Y., Yadegari, H., Agapie, T., Peters, J. C., Sargent, E. H., & Sinton, D. (2021). Cascade CO2 electroreduction enables efficient carbonate-free production of ethylene. Joule. https://doi.org/10.1016/j.joule.2021.01.007
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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