The DOI matches its Crossref record; 18 of the 18 references it cites were found in a registry or an index.
Strategies to Break the Scaling Relation toward Enhanced Oxygen Electrocatalysis
Open accessAbstract
Summary The vision of a hydrogen economy relies on efficient utilization and production of hydrogen in a hydrogen fuel cell and a water electrolyzer. In both technologies, the sluggish kinetics of oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) account for the most efficiency loss because the reactions on catalytic sites are constrained by adsorption-energy scaling relations involving intermediates of *OOH, *O, and *OH (where * denotes the active site). Therefore, a novel paradigm for catalyst design is required by overcoming or circumventing the adsorption-energy scaling relations. In this Review, the fundamentals of oxygen electrocatalysis, including reaction of the mechanism and origin of the adsorption-energy scaling relationship, are first introduced. Crucial strategies to overcome the scaling relations are then summarized. Finally, future research directions in this area are proposed. This work provides guidelines for the rational design of efficient catalysts for oxygen electrocatalysis beyond the limitation posed by scaling relations.
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Cites
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Homogeneously dispersed multimetal oxygen-evolving catalysts
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Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Defect Chemistry in Heterogeneous Catalysis: Recognition, Understanding, and Utilization
Xie, C., Yan, D., Li, H., Du, S., Chen, W., Wang, Y., Zou, Y., Chen, R., & Wang, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c03034 · Cited by 623
Sun, H., Xu, X., Kim, H., Jung, W., Zhou, W., & Shao, Z. (2023) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12441 · Cited by 601
Boosting Oxygen Electrocatalytic Activity of Fe–N–C Catalysts by Phosphorus Incorporation
Zhou, Y., Lu, R., Tao, X., Qiu, Z., Chen, G., Yang, J., Zhao, Y., Feng, X., & Müllen, K. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.2c12933 · Cited by 567
Electrocatalysis in Alkaline Media and Alkaline Membrane-Based Energy Technologies
Yang, Y., Peltier, C. R., Zeng, R., Schimmenti, R., Li, Q., Huang, X., Yan, Z., Potsi, G., Selhorst, R., Lu, X., et al. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00331 · Cited by 544
Metadata
- Authors
- Huang, Z.-F., Song, J., Dou, S., Li, X., Wang, J., & Wang, X.
- Venue
- Matter
- Publisher
- Elsevier BV
- Published
- 2019-12
- Volume
- 1
- Issue
- 6
- Pages
- 1494-1518
- ISSN
- 2590-2385 (ISSN-L)
- OpenAlex
- W2992188349
- Cited by
- 562
- References
- 18
- FWCI
- 10.31
- Type
- journal article
- Language
- en
- Open access
- bronze
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