The DOI matches its Crossref record; 158 of the 158 references it cites were found in a registry or an index.
Structural Regulation with Atomic-Level Precision: From Single-Atomic Site to Diatomic and Atomic Interface Catalysis
Open accessAbstract
Summary As a new, emerging class in catalysis field, single-atomic-site catalysts (SASCs) have displayed outstanding activities, selectivities, and stabilities in a range of important catalytic reactions. The compositions and structures of SASCs have a great impact on catalytic performances; therefore, the central task is to rationally manipulate the structures with atomic-level precision, and thereupon to design different active sites to promote the overall performances. Here, we compare SASCs with clusters/nanoparticles in term of their catalytic behaviors, and systematically interpret the impacts of the microscopic structures of SASCs on catalytic performances. Subsequently, we summarize the reports on synergistic catalysis over diatomic, multiatomic sites, single-atom alloys, and atomic interfaces, and highlight the great significance of in situ characterization technologies for monitoring the active sites. Finally, we discuss the limitations, development trends, and future challenges of SASCs, and present an outlook on further constructing more sophisticated active sites for more complex catalytic reactions.
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Cited by
Principles of Designing Electrocatalyst to Boost Reactivity for Seawater Splitting
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Metadata
- Authors
- Pan, Y., Zhang, C., Liu, Z., Chen, C., & Li, Y.
- Venue
- Matter
- Publisher
- Elsevier BV
- Published
- 2020-01
- Volume
- 2
- Issue
- 1
- Pages
- 78-110
- ISSN
- 2590-2385 (ISSN-L)
- OpenAlex
- W2999589596
- Cited by
- 341
- References
- 158
- FWCI
- 19.76
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Pan, Y., Zhang, C., Liu, Z., Chen, C., & Li, Y. (2020). Structural Regulation with Atomic-Level Precision: From Single-Atomic Site to Diatomic and Atomic Interface Catalysis. Matter. https://doi.org/10.1016/j.matt.2019.11.014
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