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Hybrid polymer/MOF membranes for Organic Solvent Nanofiltration (OSN): Chemical modification and the quest for perfection
Open accessAbstract
Abstract One of the main challenges in the field of Organic Solvent Nanofiltration (OSN) is to improve the selectivity of membranes, allowing the separation of closely related solutes. This objective might be achieved by constructing membranes with uniform porous structures. Hybrid Polymer/Metal Organic Framework (MOF) membranes were prepared by in-situ growth (ISG) of HKUST-1 within the pores of polyimide membranes. To improve the performances of ISG membranes, chemical modification was performed. Aryl carboxylic acid moieties were introduced to polyimide P84 ultrafiltration membranes allowing coordination of the HKUST-1 directly on to the polymer. Chemically modified ISG membranes outperformed non-modified ISG membranes in both solute retentions and permeance. Retentions of polystyrene solute in acetone were used to calculate theoretical pore size distributions for each of the membranes tested. It was found that the chemically modified ISG membrane had he narrowest calculated pore size distribution.
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Cites
Tempelaar, S., Mespouille, L., Coulembier, O., Dubois, P., & Dove, A. P. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35268k · Cited by 345
Cited by
Yusuf, V. F., Malek, N. I., & Kailasa, S. K. (2022) · ACS Omega · doi:10.1021/acsomega.2c05310 · Cited by 894
Metal–organic frameworks based membranes for liquid separation
Li, X., Liu, Y., Wang, J., Gascon, J., Li, J., & Van der Bruggen, B. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00575j · Cited by 747
Advances in metal–organic framework-based membranes
Cheng, Y., Datta, S. J., Zhou, S., Jia, J., Shekhah, O., & Eddaoudi, M. (2022) · Chemical Society Reviews · doi:10.1039/d2cs00031h · Cited by 423
Recent progress of organic solvent nanofiltration membranes
Shi, G. M., Feng, Y., Li, B., Tham, H. M., Lai, J.-Y., & Chung, T.-S. (2021) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2021.101470 · Cited by 280
Metadata
- Authors
- Campbell, J., Burgal, J. D. S., Szekely, G., Davies, R. P., Braddock, D. C., & Livingston, A.
- Venue
- Journal of Membrane Science
- Publisher
- Elsevier BV
- Published
- 2016-04
- Volume
- 503
- Pages
- 166-176
- ISSN
- 0376-7388 (ISSN-L)
- OpenAlex
- W2245153959
- Cited by
- 167
- References
- 1
- FWCI
- 11.38
- Type
- journal article
- Language
- en
- Open access
- green
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- Campbell, J., Burgal, J. D. S., Szekely, G., Davies, R. P., Braddock, D. C., & Livingston, A. (2016). Hybrid polymer/MOF membranes for Organic Solvent Nanofiltration (OSN): Chemical modification and the quest for perfection. Journal of Membrane Science. https://doi.org/10.1016/j.memsci.2016.01.024
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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