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Fundamental degradation mechanisms of layered oxide Li-ion battery cathode materials: Methodology, insights and novel approaches
Open accessAbstract
This overview addresses the atomistic aspects of degradation of layered LiMO2 (M = Ni, Co, Mn) oxide Li-ion battery cathode materials, aiming to shed light on the fundamental degradation mechanisms especially inside active cathode materials and at their interfaces. It includes recent results obtained by novel in situ/in operando diffraction methods, modelling, and quasi in situ surface science analysis. Degradation of the active cathode material occurs upon overcharge, resulting from a positive potential shift of the anode. Oxygen loss and eventual phase transformation resulting in dead regions are ascribed to changes in electronic structure and defect formation. The anode potential shift results from loss of free lithium due to side reactions occurring at electrode/electrolyte interfaces. Such side reactions are caused by electron transfer, and depend on the electron energy level alignment at the interface. Side reactions at electrode/electrolyte interfaces and capacity fade may be overcome by the use of suitable solid-state electrolytes and Li-containing anodes.
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Cited by
A review on the key issues of the lithium ion battery degradation among the whole life cycle
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Tran, M.-K., Mathew, M., Janhunen, S., Panchal, S., Raahemifar, K., Fraser, R., & Fowler, M. (2021) · Journal of Energy Storage · doi:10.1016/j.est.2021.103252 · Cited by 564
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Stabilizing the Interface of NASICON Solid Electrolyte against Li Metal with Atomic Layer Deposition
Liu, Y., Sun, Q., Zhao, Y., Wang, B., Kaghazchi, P., Adair, K. R., Li, R., Zhang, C., Liu, J., Kuo, L.-Y., et al. (2018) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.8b06366 · Cited by 312
Metadata
- Authors
- Hausbrand, R., Cherkashinin, G., Ehrenberg, H., Gröting, M., Albe, K., Hess, C., & Jaegermann, W.
- Venue
- Materials Science and Engineering: B
- Publisher
- Elsevier BV
- Published
- 2015-02
- Volume
- 192
- Pages
- 3-25
- ISSN
- 0921-5107 (ISSN-L)
- OpenAlex
- W1998040904
- Cited by
- 478
- References
- 8
- FWCI
- 14.50
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Hausbrand, R., Cherkashinin, G., Ehrenberg, H., Gröting, M., Albe, K., Hess, C., & Jaegermann, W. (2015). Fundamental degradation mechanisms of layered oxide Li-ion battery cathode materials: Methodology, insights and novel approaches. Materials Science and Engineering: B. https://doi.org/10.1016/j.mseb.2014.11.014
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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