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Nanoscale design of zinc anodes for high-energy aqueous rechargeable batteries

Wu, T.-H., Zhang, Y., Althouse, Z.D., Liu, N.·2019·Materials Today Nano

Abstract

Abstract Rechargeable zinc-based aqueous batteries have attracted increasing attention because of the merits of inherent safety, high capacity (820 Ah kg−1 and 5854 Ah L−1), and cost effectiveness. However, the poor rechargeability of Zn anodes limits their development in next-generation batteries, which is attributed to the dendrite growth, shape change, passivation, and hydrogen evolution issues in the zinc anodes. Nanomaterial design of Zn anodes provides a pathway to tackle these long-standing challenges to develop electrically rechargeable Zn anodes. In this review, we summarize the most recent advances, including 3D high surface area electrode structure, core/shell structure with surface coatings, and nanocomposites with highly conductive materials, in various strategies for improving zinc electrochemical performance. Additionally, the concepts of molecular design of the aqueous electrolytes with confined water molecules and high salt concentration are introduced. Finally, future opportunities and challenges with zinc-based aqueous batteries are discussed.

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Metadata

Authors
Wu, T.-H., Zhang, Y., Althouse, Z. D., & Liu, N.
Venue
Materials Today Nano
Publisher
Elsevier BV
Published
2019-06
Volume
6
Pages
100032
ISSN
2588-8420 (ISSN-L)
OpenAlex
W2927323160
Cited by
190
References
1
FWCI
10.22
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Nanoscale design of zinc anodes for high-energy aqueous rechargeable batteries. https://app.cochat.ai/papers/10.1016/j.mtnano.2019.100032
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Wu, T.-H., Zhang, Y., Althouse, Z. D., & Liu, N. (2019). Nanoscale design of zinc anodes for high-energy aqueous rechargeable batteries. Materials Today Nano. https://doi.org/10.1016/j.mtnano.2019.100032

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