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Cited by 32Laser Material Processing TechniquesUltrasound and Cavitation PhenomenaLaser-Ablation Synthesis of Nanoparticles

Dynamics of laser-induced cavitation bubble during expansion over sharp-edge geometry submerged in liquid – an inside view by diffuse illumination

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Senegačnik, Matej, Kunimoto, Kohei, Yamaguchi, Satoshi, Kimura, Koki, Sakka, Tetsuo, Gregorčič, Peter·2021·Ultrasonics Sonochemistry
DOI 10.1016/j.ultsonch.2021.105460PMC PMC8027904
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Abstract

Laser ablation in liquids is growing in popularity for various applications including nanoparticle production, breakdown spectroscopy, and surface functionalization. When laser pulse ablates the solid target submerged in liquid, a cavitation bubble develops. In case of “finite” geometries of ablated solids, liquid dynamical phenomena can occur inside the bubble when the bubble overflows the surface edge. To observe this dynamics, we use diffuse illumination of a flashlamp in combination with a high-speed videography by exposure times down to 250 ns. The developed theoretical modelling and its comparison with the experimental observations clearly prove that this approach widens the observable area inside the bubble. We thereby use it to study the dynamics of laser-induced cavitation bubble during its expansion over a sharp-edge (“cliff-like” 90°) geometry submerged in water, ethanol, and polyethylene glycol 300. The samples are 17 mm wide stainless steel plates with thickness in the range of 0.025–2 mm. Bubbles are induced on the samples by 1064-nm laser pulses with pulse durations of 7–60 ns and pulse energies of 10–55 mJ. We observe formation of a fixed-type secondary cavity behind the edge where low-pressure area develops due to bubble-driven flow of the liquid. This occurs when the velocity of liquid overflow exceeds ~20 m s−1. A re-entrant liquid injection with up to ~40 m s−1 velocity may occur inside the bubble when the bubble overflows the edge of the sample. Formation and characteristics of the jet evidently depend on the relation between the breakdown-edge offset and the bubble energy, as well as the properties of the surrounding liquid. Higher viscosity of the liquid prevents the generation of the jet.

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  • Senegačnik et al. demonstrated that using diffused illumination technique, fluid dynamics of bubble growth, expansion, and shrinkage can be examined more accurately.

    “Senegačnik et al. [83] demonstrated that using the diffused illumination technique, the fluid dynamics of the bubble growth, expansion, and shrinkage can be examined more accurately.”

    From Influence of Laser Process Parameters, Liquid Medium, and External Field on the Synthesis of Colloidal Metal Nanoparticles Using Pulsed Laser Ablation in Liquid: A Review (2022) · cites this paper as [83]

    The Introduction and ‘Role of illumination diffusivity in bubble imaging’ (pages not provided) say diffuse illumination widens the visible area inside a cavitation bubble, enabling high-resolution observation of internal liquid dynamics during expansion. They do not establish more accurate examination of bubble growth and shrinkage generally; the imaging section cautions that diffuse illumination can blur the bubble wall and affect apparent bubble size. (LLM, conf=0.86)

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Authors
Senegačnik, M., Kunimoto, K., Yamaguchi, S., Kimura, K., Sakka, T., & Gregorčič, P.
Affiliations
  • University of Ljubljana (SI)
  • Kyoto University (JP)
Corresponding author
Gregorčič, Peter
ORCID
Venue
Ultrasonics Sonochemistry
Publisher
Elsevier BV
Published
2021-05
Volume
73
Pages
105460
ISSN
1350-4177 (ISSN-L)
DOI
10.1016/j.ultsonch.2021.105460
PMC
PMC8027904
OpenAlex
W3119903432
Cited by
32
References
3
Citations by year
2026: 8 · 2025: 5 · 2024: 7 · 2023: 4 · 2022: 6 · 2021: 2
FWCI
2.70
Type
journal article
Language
en
Open access
Licence
Locations
  • Ultrasonics Sonochemistry (publishedVersion, cc-by)
  • PubMed Central (publishedVersion, cc-by)
  • PubMed (publishedVersion)
  • Repository of the University of Ljubljana (University of Ljubljana) (publishedVersion, cc-by)
  • dCOBISS.SI Digital Repository (submittedVersion, cc-by)
  • DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
Funders
  • Javna Agencija za Raziskovalno Dejavnost RS (BI-JP/18-20-004, J2-1741, P2-0392)
  • Japan Society for the Promotion of Science (JP20H02764)
Topics
  • Physical Sciences › Engineering › Computational Mechanics › Laser Material Processing Techniques
  • Physical Sciences › Materials Science › Materials Chemistry › Ultrasound and Cavitation Phenomena
  • Physical Sciences › Engineering › Biomedical Engineering › Laser-Ablation Synthesis of Nanoparticles
Keywords
laser-induced cavitation, cavitation bubble dynamics, liquid jet formation, re-entrant jet, bubble-driven flow, liquid viscosity effects, stainless steel target, diffuse illumination, high-speed video, water, ethanol, polyethylene glycol

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