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Selective Diagnosis of Diabetes Using Pt-Functionalized WO3 Hemitube Networks As a Sensing Layer of Acetone in Exhaled Breath
Abstract
Thin-walled WO(3) hemitubes and catalytic Pt-functionalized WO(3) hemitubes were synthesized via a polymeric fiber-templating route and used as exhaled breath sensing layers for potential diagnosis of halitosis and diabetes through the detection of H(2)S and CH(3)COCH(3), respectively. Pt-functionalized WO(3) hemitubes with wall thickness of 60 nm exhibited superior acetone sensitivity (R(air)/R(gas) = 4.11 at 2 ppm) with negligible H(2)S response, and pristine WO(3) hemitubes showed a 4.90-fold sensitivity toward H(2)S with minimal acetone-sensing characteristics. The detection limit (R(air)/R(gas)) of the fabricated sensors with Pt-functionalized WO(3) hemitubes was 1.31 for acetone of 120 ppb, and pristine WO(3) hemitubes showed a gas response of 1.23 at 120 ppb of H(2)S. Long-term stability tests revealed that the remarkable selectivity has been maintained after aging for 7 months in air. The superior cross-sensitivity and response to H(2)S and acetone gas offer a potential platform for application in diabetes and halitosis diagnosis.
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Cited by
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Li, G., Cheng, Z., Xiang, Q., Yan, L., Wang, X., & Xu, J. (2019) · Sensors and Actuators B: Chemical · doi:10.1016/j.snb.2018.09.117 · Cited by 422
Functional gas sensing nanomaterials: A panoramic view
Malik, R., Tomer, V. K., Mishra, Y. K., & Lin, L. (2020) · Applied Physics Reviews · doi:10.1063/1.5123479 · Cited by 410
Yang, G., Li, X., He, Y., Ma, J., Ni, G., & Zhou, S. (2018) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2017.12.003 · Cited by 336
Prospects and Challenges of Volatile Organic Compound Sensors in Human Healthcare
Jalal, A. H., Alam, F., Roychoudhury, S., Umasankar, Y., Pala, N., & Bhansali, S. (2018) · ACS Sensors · doi:10.1021/acssensors.8b00400 · Cited by 315
Innovative Nanosensor for Disease Diagnosis
Kim, S.-J., Choi, S.-J., Jang, J.-S., Cho, H.-J., & Kim, I.-D. (2017) · Accounts of Chemical Research · doi:10.1021/acs.accounts.7b00047 · Cited by 264
Self-citationPeng, B., Zhao, F., Ping, J., & Ying, Y. (2020) · Small · doi:10.1002/smll.202002681 · Cited by 224
Li, T., Yin, W., Gao, S., Sun, Y., Xu, P., Wu, S., Kong, H., Yang, G., & Wei, G. (2022) · Nanomaterials · doi:10.3390/nano12060982 · Cited by 222
Electronic nose: a non-invasive technology for breath analysis of diabetes and lung cancer patients
Behera, B., Joshi, R., Anil Vishnu, G. K., Bhalerao, S., & Pandya, H. J. (2019) · Journal of Breath Research · doi:10.1088/1752-7163/aafc77 · Cited by 179
Metadata
- Authors
- Choi, S.-J., Lee, I., Jang, B.-H., Youn, D.-Y., Ryu, W.-H., Park, C. O., & Kim, I.-D.
- Venue
- Analytical Chemistry
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-01-07
- Volume
- 85
- Issue
- 3
- Pages
- 1792-1796
- ISSN
- 0003-2700 (ISSN-L)
- 1520-6882
- OpenAlex
- W2329751486
- Cited by
- 311
- References
- 0
- FWCI
- 9.56
- Type
- journal article
- Language
- en
- Open access
- closed
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